Multiple charge density wave ordering and quantum coupling of collective excitations in layered
Phys. Rev. B 110, 075155 – Published 27 August, 2024
DOI: https://doi.org/10.1103/PhysRevB.110.075155
Abstract
Rare-earth tritellurides represent quasi-two-dimensional systems that exhibit multiple charge density wave (CDW) transitions alongside magnetic ordering. However, the interplay between the phonon dynamics of collective excitations and local magnetism remains unclear. is an interesting material having an incommensurate CDW (ICDW), at K, an antiferromagnetic transition at K, and with an expectation of another CDW ordering. We emphasize electron-spin-phonon and mode coupling in through temperature dependent Raman spectroscopy complemented by heat capacity and magnetization measurements. Disappearance of zone-folded mode (Z*) and observed coupling behavior of amplitude mode suggest the existence of another ordering at K, in addition to known ICDW. By employing phonon renormalization, we estimated significant strength of spin-phonon coupling, and accentuated on the phonon dynamics associated with CDW instabilities in .