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  • Letter

Quantum impurity model for two-stage multipolar ordering and Fermi surface reconstruction

Daniel J. Schultz*, SangEun Han*, and Yong Baek Kim

  • Department of Physics, University of Toronto, Toronto, Ontario M5S 1A7, Canada

  • *These authors contributed equally to this work.

Phys. Rev. B 108, L060401 – Published 8 August, 2023

DOI: https://doi.org/10.1103/PhysRevB.108.L060401

Abstract

Classification and understanding of quantum phase transitions and critical phenomena in itinerant electron systems are outstanding questions in quantum materials research. Recent experiments on heavy fermion systems with higher-rank multipolar local moments provide a new platform to study such questions. In particular, experiments on Ce3Pd20(Si,Ge)6 show novel quantum critical behaviors via two consecutive magnetic field-driven quantum phase transitions. At each transition, the derivative of the Hall resistivity jumps discontinuously, which was attributed to sequential Fermi surface reconstructions. Motivated by this discovery, we consider an effective quantum impurity model of itinerant electrons coupled to local dipolar, quadrupolar, and octupolar moments arising from Ce3+ ions. Using renormalization group analyses, we demonstrate that two-stage multipolar ordering and Fermi surface reconstruction arise depending on which multipolar moments participate in the Fermi surface and which other moments are decoupled via Kondo destruction.

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