• Accepted Paper

Comprehensive frequency- and time-domain investigation of coherent exciton dynamics in strained GaAs films

Samia Alyami, Matthew T. Larson, Vermilion Villarreal, Heidrun Schmitzer, Tuomas Haggren, Hark Hoe Tan, Chennupati Jagadish, and Hans Peter Wagner

Phys. Rev. B - Accepted 8 October, 2026

DOI: https://doi.org/10.1103/yyyb-7cvf

Abstract

In this study, we investigate coherent exciton dynamics in a thin GaAs film using three-beam four-wave mixing (FWM) techniques. The GaAs film exhibits spatially varying biaxial tensile strain, enabling us to study the influence of differing strain on the dephasing time of strain-split heavy- and light-hole excitons. Heterodyne FWM experiments reveal an essentially homogeneously broadened exciton polarization throughout the film. While the exciton dephasing rates show no discernible correlation with the local strain variations, excitation-induced dephasing becomes the dominant FWM generation process at long dephasing times. Under cross-linear excitation the FWM signal mainly originates from two-exciton correlations. Theoretical analysis using the 10-level optical Bloch equations substantiates these findings. The strain resilience of the picosecond-scale exciton dephasing time suggests GaAs films as a powerful platform for investigating coherent light-matter interactions and coupling in composite exciton-plasmon quantum systems.

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