• Accepted Paper

Collapse of the Shastry-Sutherland lattice in TmB4 under tilted magnetic fields

Matúš Orendáč, Slavomír Gabáni, Gabriel Pristáš, Július Bačkai, Konrad Siemensmeyer, Karel Prokeš, Natalya Shitsevalova, Yurii Skourski, and Karol Flachbart

Phys. Rev. B - Accepted 9 October, 2026

DOI: https://doi.org/10.1103/pwyz-x5l6

Abstract

The two-dimensional Shastry-Sutherland lattice (SSL) belongs to important models in the field of quantum magnetism as it combines low-dimensionality, geometrical frustration and strong anisotropy. Besides the insulating SrCu₂(BO₃)₂, the metallic tetraboride TmB4 belongs to its best-known examples. In this work, we investigate the development of TmB4 magnetization under magnetic fields (B) up to 60 T, applied at different angles with respect to the easy magnetization axis c. We aim to determine the extent to which phenomena associated with the SSL remain robust in high magnetic fields when the field is tilted away from this direction. Our results show that at temperatures (T) below 20 K significant deviations from the easy-axis interpretation of magnetization, in which the magnetic moments of Tm-ions are oriented only parallel to c axis, occur at deflection angles higher than 70 degree and in magnetic fields above 30 T. These values noticeably affect the corresponding B vs T phase diagram of TmB4 and point to a collapse of SSL phenomena under these conditions. The observed high field magnetization anomalies in TmB4 may also suggest the existence of new field induced quantum phases in this Shastry-Sutherland compound.

Export citation

Export citation

Choose format for download:

Download Citation

If the author has provided any supplemental materials with this article they will be available upon publication of the version of record.

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation