- Accepted Paper
Dynamical magnetism in the disordered cubic lattice material -BaCoNbO
Phys. Rev. B - Accepted 22 September, 2026
DOI: https://doi.org/10.1103/jsvt-jc4l
Phys. Rev. B - Accepted 22 September, 2026
DOI: https://doi.org/10.1103/jsvt-jc4l
- realizes a disordered simple-cubic spin- lattice in which Co ions randomly occupy one-third of the sites, placing the system just above the site-percolation threshold for magnetic order. Specific-heat, susceptibility, neutron spin-echo, and muon spin-rotation measurements reveal a broad thermodynamic crossover, short-range magnetic correlations, and persistent fast spin dynamics down to at least 0.1 K, with no evidence for static order or conventional spin-glass freezing within the experimental time windows. Monte Carlo simulations yield a broad distribution of orphan spins, finite clusters, and an infinite network. The weakly correlated spin fraction () inferred phenomenologically from magnetization is consistent with the calculated orphan-spin fraction (). Exact diagonalization of a diluted Heisenberg model captures the broad magnetic specific-heat anomaly and supports the coexistence of weakly and strongly correlated spin environments. These results support a picture in which spin- quantum fluctuations, together with dilution and proximity to the percolation threshold, can support a disorder-driven dynamical state with short-range correlations in three dimensions, distinct from both classical spin glasses and geometrically frustrated quantum spin liquids.
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