- Editors' Suggestion
- Letter
Three-dimensional zigzag correlations in the van der Waals Kitaev magnet
Phys. Rev. B 114, L140404 – Published 10 September, 2026
DOI: https://doi.org/10.1103/zwvv-5594
Abstract
Ruthenium trihalides () provide a tunable platform for Kitaev magnetism in two-dimensional van der Waals materials. Despite their similar crystal structures and zigzag antiferromagnetic order, exhibits a higher Néel temperature () than , suggesting their distinct proximity to the Kitaev quantum spin-liquid phase. Using Ru -edge resonant x-ray scattering, we show that, while the long-range zigzag order in disappears at , the zigzag correlations that persist well above show a pronounced spectral weight redistribution along the interlayer direction. These results suggest that the enhanced interlayer magnetic interactions driven by the extended Br orbitals stabilize three-dimensional zigzag correlations in .