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Three-dimensional zigzag correlations in the van der Waals Kitaev magnet RuBr3

H. Gretarsson1,*, R. Iwazaki2, F. Sato2, H. Gotou3, S. Francoual1, J. Nasu2, Y. Imai2,4, K. Ohgushi2, J. Chaloupka5 et al.

B. Keimer6 and H. Suzuki7,8,†

  • *Contact author: hlynur.gretarsson@desy.de
  • †Contact author: hakuto.suzuki@tohoku.ac.jp

Phys. Rev. B 114, L140404 – Published 10 September, 2026

DOI: https://doi.org/10.1103/zwvv-5594

Abstract

Ruthenium trihalides RuX3 (X=Cl,Br,I) provide a tunable platform for Kitaev magnetism in two-dimensional van der Waals materials. Despite their similar crystal structures and zigzag antiferromagnetic order, RuBr3 exhibits a higher Néel temperature (TN) than RuCl3, suggesting their distinct proximity to the Kitaev quantum spin-liquid phase. Using Ru L3-edge resonant x-ray scattering, we show that, while the long-range zigzag order in RuBr3 disappears at TN, the zigzag correlations that persist well above TN show a pronounced spectral weight redistribution along the interlayer direction. These results suggest that the enhanced interlayer magnetic interactions driven by the extended Br 4p orbitals stabilize three-dimensional zigzag correlations in RuBr3.

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