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    Magnetic field and pressure tuning of the heavy fermion antiferromagnet CePdIn

    Bin Shen1,*,†, Feng Du1,‡, Rui Li1, Hang Su1,§, Yasuyuki Shimura2, Takahiro Onimaru2, Kazunori Umeo3, Xin Lu1, Toshiro Takabatake1,2 et al.

    Michael Smidman1,∥ and Huiqiu Yuan1,4,5,6,¶

    • 1New Cornerstone Science Laboratory, Center for Correlated Matter and School of Physics, Zhejiang University, Hangzhou 310058, China
    • 2Department of Quantum Matter, Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima 739-8530, Japan
    • 3Department of Low Temperature Experiment, Integral Experimental Support/Research Division, N-BARD, Hiroshima University, Higashi-Hiroshima 739-8526, Japan
    • 4Institute for Advanced Study in Physics, Zhejiang University, Hangzhou 310058, China
    • 5Institute of Fundamental and Transdisciplinary Research, Zhejiang University, Hangzhou 310058, China
    • 6State Key Laboratory of Silicon and Advanced Semiconductor Materials, Zhejiang University, Hangzhou 310058, China

    • *Contact author: bin.shen@physik.uni-augsburg.de
    • †Present address: Experimental Physics VI, Center for Electronic Correlations and Magnetism, University of Augsburg, 86159 Augsburg, Germany.
    • ‡Present address: Max Planck Institute for Chemistry, Hahn Meitner Weg 1, Mainz 55128, Germany.
    • §Present address: Department of Physics, University of Tokyo, Bunkyo-ku, Tokyo, Japan.
    • ∥Contact author: msmidman@zju.edu.cn
    • Contact author: hqyuan@zju.edu.cn

    Phys. Rev. B 113, 115130 – Published 13 March, 2026

    DOI: https://doi.org/10.1103/zvp2-gq4m

    Abstract

    Frustrated Kondo lattices are ideal platforms for studying how both the Kondo effect and quantum fluctuations compete with the magnetic exchange interactions that drive magnetic ordering. Here, we investigate the effect of tuning the heavy-fermion compound CePdIn, which crystallizes in the geometrically frustrated ZrNiAl-type structure, using applied magnetic fields and hydrostatic pressure. At ambient pressure, CePdIn exhibits two magnetic transitions, one at TN≈1.65K and another at TM≈1.15K, which are both suppressed by applied c-axis fields. Upon applying pressure in zero magnetic field, there is a nonmonotonic evolution of TN, which decreases to 0.8 K at 2.3 GPa, before abruptly increasing to 1.5 K at 2.6 GPa. At higher pressures, TN has a weak pressure dependence and vanishes near 5 GPa. Together with the high-pressure phase being more robust to applied fields, these results suggest two distinct antiferromagnetic phases in CePdIn, which are separated near 2.6 GPa, and this change may be driven by the evolution of the underlying electronic structure due to enhanced Kondo hybridization under pressure.

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