Strain-stabilized high-topological-charge skyrmions and field-tunable phase switching in frustrated monolayer
Phys. Rev. B 113, 024404 – Published 5 January, 2026
DOI: https://doi.org/10.1103/ztd2-449j
Abstract
Monolayer exhibits strain-tunable topological magnetism mediated by competing exchange interactions on a triangular lattice. Our first-principles calculations show biaxial strain () controls both the exchange frustration strength and magnetic anisotropy energy, with Br-driven spin-orbit coupling flipping the magnetic easy axis at . In addition, the spin dynamics simulations reveal how strain-enhanced frustration nucleates domain walls that fragment into high-topological-charge skyrmions () under out-of-plane magnetic fields. Deterministic switching between skyrmions and bimeron pairs textures emerges via coordinated in-plane/out-of-plane magnetic fields, while a universal topological collapse beyond a magnetic field T confirms Zeeman energy dominance. This strain-frustration-anisotropy interplay establishes a control paradigm for exotic spin topologies in two-dimensional magnets.