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    Strain-stabilized high-topological-charge skyrmions and field-tunable phase switching in frustrated monolayer NiBr2

    Zhen Sun, Shiwei Zhu, Xinyuan Guan, Xiaoping Wu, and Changsheng Song*

    • Zhejiang Key Laboratory of Quantum State Control and Optical Field Manipulation, Department of Physics, Zhejiang Sci-Tech University, 310018 Hangzhou, China

    • *Contact author: cssong@zstu.edu.cn

    Phys. Rev. B 113, 024404 – Published 5 January, 2026

    DOI: https://doi.org/10.1103/ztd2-449j

    Abstract

    Monolayer NiBr2 exhibits strain-tunable topological magnetism mediated by competing exchange interactions on a triangular lattice. Our first-principles calculations show biaxial strain (ɛ) controls both the exchange frustration strength η=|J1/J3| and magnetic anisotropy energy, with Br-driven spin-orbit coupling flipping the magnetic easy axis at ɛ=2%. In addition, the spin dynamics simulations reveal how strain-enhanced frustration nucleates domain walls that fragment into high-topological-charge skyrmions (Q>1) under out-of-plane magnetic fields. Deterministic switching between skyrmions and bimeron pairs textures emerges via coordinated in-plane/out-of-plane magnetic fields, while a universal topological collapse beyond a magnetic field B>1.8 T confirms Zeeman energy dominance. This strain-frustration-anisotropy interplay establishes a control paradigm for exotic spin topologies in two-dimensional magnets.

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