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    Reexamining the strange metal charge response with transmission inelastic electron scattering

    Niels de Vries1,2,*, Eric Hoglund3,†, Dipanjan Chaudhuri1,2, Sang hyun Bae1,4, Jin Chen1,2, Xuefei Guo1,2, David Bałut1,2, Genda Gu5, Pinshane Huang1,4 et al.

    Jordan Hachtel3 and Peter Abbamonte1,2,‡

    • 1Materials Research Laboratory, Grainger College of Engineering, University of Illinois, Urbana-Champaign, 104 S. Goodwin Ave., Urbana, Illinois 61801, USA
    • 2Department of Physics, Grainger College of Engineering, University of Illinois, Urbana-Champaign, 1110 W. Green St., Urbana, Illinois 61801, USA
    • 3Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA
    • 4Department of Materials Science and Engineering, Grainger College of Engineering, University of Illinois, Urbana-Champaign, 1110 W. Green St., Urbana, Illinois 61801, USA
    • 5Division of Condensed Matter Physics and Materials Science, Brookhaven National Laboratory, Upton, New York 11973, USA

    • *Contact author: niels@illinois.edu
    • †Contact author: hoglunder@ornl.gov
    • ‡Contact author: abbamont@illinois.edu

    Phys. Rev. B 113, 235158 – Published 30 June, 2026

    DOI: https://doi.org/10.1103/zp4x-r2jk

    Abstract

    The strange metal remains a major unsolved problem for modern condensed matter physics. Since the early development of marginal Fermi liquid phenomenology, it has been clear that progress requires detailed knowledge of the momentum- and frequency-dependent charge susceptibility χ(q,ω), particularly at large momenta. Electron energy-loss spectroscopy (EELS), performed in either reflection or transmission geometry, provides the most direct probe of χ(q,ω). However, measurements over the past four decades have yielded conflicting results, with authors of some studies reporting a dispersing random phase approximation (RPA)-like plasmon and others observing a strongly overdamped, incoherent response. Here, we report a transmission EELS study of Bi2Sr2CaCu2O8+x (Bi-2212) that simultaneously achieves high-energy resolution (ΔE≈30meV) and high-momentum resolution (Δq≈0.01Å−1). To address issues of reproducibility, measurements were repeated 10 times on five different Bi-2212 flakes, benchmarked against aluminum, a well-characterized Fermi liquid, and quantitatively compared with those of prior studies spanning four decades. At momenta q<0.15Å−1, we observe a highly damped plasmon whose linewidth is comparable with its energy. At larger momenta q>0.15Å−1, this excitation does not disperse but instead evolves into an incoherent continuum, with no evidence for the RPA-like dispersion reported in some earlier works. Comparison with recent resonant inelastic x-ray scattering measurements on Bi-based cuprates supports the view that Bi-2212 is an incoherent metal with strongly damped charge excitations.

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