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Codimension-two spiral spin liquid in the effective honeycomb-lattice compound Cs3Fe2Cl9

Shang Gao1,2,3,*, Chris Pasco2, Otkur Omar1, Qiang Zhang3, Daniel M. Pajerowski3, Feng Ye3, Matthias Frontzek3, Andrew F. May2, Matthew B. Stone3,† et al.

Andrew D. Christianson2,‡

  • *Contact author: sgao@ustc.edu.cn
  • †Contact author: stonemb@ornl.gov
  • ‡Contact author: christiansad@ornl.gov

Phys. Rev. B 113, L140401 – Published 1 April, 2026

DOI: https://doi.org/10.1103/zm32-s2xz

Abstract

A codimension-two spiral spin liquid is a correlated paramagnetic state with one-dimensional ground state degeneracy hosted within a three-dimensional lattice. Here, via neutron scattering experiments and numerical simulations, we establish the existence of a codimension-two spiral spin liquid in the effective honeycomb-lattice compound Cs3Fe2Cl9, which demonstrates an alternate path to spiral spin liquids by overcoming the long-standing impediment of weak further-neighbor interactions. In the long-range ordered regime, competing spiral and spin density wave orders emerge as a function of applied magnetic field, among which a possible order-by-disorder transition is identified.

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