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    Intrinsic antiferromagnetic skyrmions and their strain modulation in atomically thin Janus vanadium dihalides

    Chuyu Li1, Wenzhe Zhou1,*, Yating Li1, Xianjuan He1, Yahan Chen1, and Fangping Ouyang1,2,3,†

    • 1School of Physics, Institute of Quantum Physics, Hunan Key Laboratory for Super-Microstructure and Ultrafast Process, and Hunan Key Laboratory of Nanophononics and Devices, Central South University, Changsha 410083, People's Republic of China
    • 2School of Physics and Technology, State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources, Xinjiang University, Urumqi 830046, People's Republic of China
    • 3State Key Laboratory of Powder Metallurgy, and Powder Metallurgy Research Institute, Central South University, Changsha 410083, People's Republic of China

    • *Contact author: csuzwz24@csu.edu.cn
    • †Contact author: ouyangfp06@tsinghua.org.cn

    Phys. Rev. B 112, 014424 – Published 14 July, 2025

    DOI: https://doi.org/10.1103/zhb1-5dky

    Abstract

    Two-dimensional (2D) materials hosting antiferromagnetic skyrmions are promising candidates for next-generation small-scale skyrmionic storage devices. However, the realization of antiferromagnetic skyrmions in intrinsic 2D materials, particularly in the widely studied MA2-like (M = transition metals; A = chalcogen or halogen elements) materials, remains elusive. Here, we theoretically demonstrate the emergence and strain modulation of 2D antiferromagnetic skyrmion crystal (AF-SkX) in Janus V-based dihalides VXY (X,Y=Cl,Br,I;X≠Y). The interplay between antiferromagnetic exchange and Dzyaloshinskii-Moriya interaction (DMI) gives rise to the AF-SkX phase in VXI, which consists of three antiferromagnetically coupled skyrmion crystals. Furthermore, tensile strain significantly reduces the effective magnetic field strength required to realize AF-SkX and broadens the field range over which AF-SkX appears, increasing both the feasibility and stability of AF-SkX in VClI. Our findings expand the family of 2D materials capable of hosting AF-SkX and provide perspectives for engineering antiferromagnetic skyrmions in 2D materials.

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