Intrinsic antiferromagnetic skyrmions and their strain modulation in atomically thin Janus vanadium dihalides
Phys. Rev. B 112, 014424 – Published 14 July, 2025
DOI: https://doi.org/10.1103/zhb1-5dky
Abstract
Two-dimensional (2D) materials hosting antiferromagnetic skyrmions are promising candidates for next-generation small-scale skyrmionic storage devices. However, the realization of antiferromagnetic skyrmions in intrinsic 2D materials, particularly in the widely studied -like ( = transition metals; = chalcogen or halogen elements) materials, remains elusive. Here, we theoretically demonstrate the emergence and strain modulation of 2D antiferromagnetic skyrmion crystal (AF-SkX) in Janus V-based dihalides . The interplay between antiferromagnetic exchange and Dzyaloshinskii-Moriya interaction (DMI) gives rise to the AF-SkX phase in , which consists of three antiferromagnetically coupled skyrmion crystals. Furthermore, tensile strain significantly reduces the effective magnetic field strength required to realize AF-SkX and broadens the field range over which AF-SkX appears, increasing both the feasibility and stability of AF-SkX in VClI. Our findings expand the family of 2D materials capable of hosting AF-SkX and provide perspectives for engineering antiferromagnetic skyrmions in 2D materials.