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Insight into spin-to-charge conversion in rutile RuO2

Yanzhang Cao1,*, Da Tian2,*, Lin Huang1,3, Hua Bai1, Shixuan Liang1, Lei Han1, Chong Chen1, Yichi Zhang1, Lei Wang4 et al.

Caihong Zhang2,†, Feng Pan1, Biaobing Jin2, and Cheng Song1,‡

  • 1Key Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China
  • 2Research Institute of Superconductor Electronics (RISE), School of Electronic Science and Engineering, Nanjing University, Nanjing 210023, China
  • 3Anhui Provincial Key Laboratory of Magnetic Functional Materials and Devices School of Materials Science and Engineering, Anhui University, Hefei, Anhui 230601, China
  • 4Department of Physics, Institute of Theoretical Physics, University of Science and Technology Beijing, Beijing 100083, China

  • *These authors contributed equally to this work.
  • †Contact author: chzhang@nju.edu.cn
  • ‡Contact author: songcheng@mail.tsinghua.edu.cn

Phys. Rev. B 112, 064415 – Published 7 August, 2025

DOI: https://doi.org/10.1103/z478-fgl8

Abstract

The interconversion between spin and charge current lies at the core of spintronics. Although significant efforts have been made in the study of spin-to-charge conversion, a close observation of the dynamical process of spin-to-charge remains elusive. Here we explored RuO2 film thickness-dependent terahertz (THz) emission from the ultrafast charge current converted from z spins, which are generated by incident circularly polarized lasers via optical orientation. The shift trend of the THz peak position with respect to the film thickness reveals that the conversion process occurs simultaneously with the z spin propagation within the film, rather than at the RuO2 surface. A qualitative model of spin-to-charge conversion in RuO2 was employed to explain the shift trend, fitting the experimental data with numerical calculation. Our work not only helps improve the fundamental knowledge of spin-to-charge conversion, but also advances the development of z spin-based ultrafast spintronic devices.

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