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    SU(N) spin-phonon simulations of Floquet dynamics in spin S>12 Mott insulators

    Ruairidh Sutcliffe1,*, Kathleen Hart1,*, Gil Refael2,3, and Arun Paramekanti1

    • *These authors contributed equally to this work.

    Phys. Rev. B 112, 014413 – Published 8 July, 2025

    DOI: https://doi.org/10.1103/yzwr-4d9z

    Abstract

    The dynamics of magnetic moments coupled to phonons is of great interest for understanding spin transport in solids as well as for our ability to control magnetism via tailored phonon modes. For spin S>12, spin-orbit coupling permits an unusual linear coupling of phonons to quadrupolar moments, so that phonons act as a dynamical transverse field for the spins. Here, we develop a generalized SU(N) spin-phonon Monte Carlo and molecular dynamics technique to simulate the equilibrium and nonequilibrium properties of such spin-orbital-phonon coupled Mott insulators, and apply it to a spin-1 model with competing XY antiferromagnet (AFM) and quadrupolar paramagnet (QPM) phases. We uncover a rich set of nonequilibrium phenomena from driven phonons, including the generation of a uniform magnetization in the QPM and AFM, strengthening of Néel order, gapping of the AFM Nambu-Goldstone mode by Floquet-Ising anisotropy, and creating Floquet copies of transverse and longitudinal spin waves. Our work is relevant for driven spin-1 magnets, such as Ba2FeSi2O7, and we highlight broader implications for nonequilibrium multipolar magnetism.

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