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Spin texture of α−GeTe in the ultrathin regime

Calvin Tagne-Kaegom1, Alexandre Llopez2, Boris Croes2,*, Geoffroy Kremer1, Bertrand Kierren1, Daniel Malterre1, Luc Moreau1, Fotié Jaurès Ngoufo2, Stefano Curiotto2 et al.

Pierre Müller2, Patrick Le Fèvre3,‡, Julien Rault3, François Bertran3, Andrés Saúl2, Frédéric Leroy2, Fabien Cheynis2,†, and Yannick Fagot-Revurat1

  • *Present address: Université de Strasbourg, CNRS, IPCMS, UMR 7504, F-67000 Strasbourg, France.
  • †Contact author: fabien.cheynis@univ-amu.fr
  • ‡Present address: Université Rennes, IPR, UMR 6251, CNRS, F-35000 Rennes, France.

Phys. Rev. B 113, 125113 – Published 9 March, 2026

DOI: https://doi.org/10.1103/yst7-ktp9

Abstract

Using spin- and angle-resolved photoemission spectroscopy combined with density functional theory calculations, we investigate the electronic structure of α-GeTe grown on a Si(111)-Sb substrate in the ultrathin limit. The full band structure, including the Fermi surface, and spin texture characterizations are presented, with a focus on a film thickness of 5 nm. Well-defined spin-polarized quantum well bulk states are evidenced. This confirms the high quality of elaborated ultrathin films and allows precise determination of the thickness. The Rashba splitting and the in-plane spin texture of GeTe bulk bands are shown to be fully preserved on the Si(111)-Sb substrate. This suggests the persistence of inversion symmetry breaking and ferroelectric properties in the ultrathin limit of GeTe films. Our results demonstrate that device downscaling can be pursued in the context of all-electrically controlled spin-orbitronics applications.

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