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Hund's coupling governed orbital-selective superconductivity in Ba1−xKxFe2As2

Elena Corbae1,2,3,*, Rong Zhang1,2, Cong Li4, Kunihiro Kihou5, Chul-Ho Lee5, Makoto Hashimoto6, Thomas Devereaux1,7, Oscar Tjernberg4, Egor Babaev8,9 et al.

Dung-Hai Lee10,11, Vadim Grinenko12, Donghui Lu6,†, and Zhi-Xun Shen1,2,3,13,‡

  • *Contact author: ecorbae@stanford.edu
  • †Contact author: dhlu@slac.stanford.edu
  • ‡Contact author: zxshen@stanford.edu

Phys. Rev. B 113, 224517 – Published 12 June, 2026

DOI: https://doi.org/10.1103/yry8-qdm6

Abstract

Understanding how strong electronic correlations shape superconductivity remains a central challenge in quantum materials. In multiorbital systems, correlations driven by Hund's coupling can differentiate the behavior of individual orbitals, producing the so-called Hund's metal state. How such orbital-selectivity also governs superconducting pairing, however, has remained largely unexplored experimentally. Here we use high-resolution angle-resolved photoemission spectroscopy to systematically map the superconducting gap structure across the phase diagram of the representative iron-based superconductor Ba1−xKxFe2As2. We find that superconductivity evolves in a strongly orbital-dependent manner: the gap associated with the dxy orbital collapses beyond optimal doping while pairing on the dxz/dyz orbitals persists. This behavior mirrors the orbital-selective correlations observed in the normal state and reveals a direct connection between Hund's metal physics and the superconducting pairing landscape. Our results demonstrate that superconducting gaps themselves can serve as a sensitive probe of orbital-dependent correlations and suggest that Hund's coupling plays a central role in shaping pairing in multiorbital superconductors.

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