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    Antiferromagnetic resonance and two-magnon absorption in an XXZ-chain antiferromagnet Cs2CoCl4

    Phys. Rev. B 112, 174421 – Published 17 November, 2025

    DOI: https://doi.org/10.1103/ynvv-tszv

    Abstract

    Magnetic excitations of the exchange-dipole quasi-one-dimensional XXZ antiferromagnet are studied in the ordered phase. We observe a transformation of the electron spin resonance (ESR) spectrum when crossing the Néel temperature near 0.2 K. The single-mode ESR of a correlated XXZ chain transforms in the multimode spectrum in the ordered phase. The multimode spectrum consists mainly of the intensive mode of a single correlated chain, which is surrounded and/or indented by numerous weak satellites. The number of securely fixed modes is eight at H∥b and twelve at H∥a. In addition to the multimode resonance observed at the transverse polarization of the microwave and static magnetic fields, we reveal a wide band of absorption by (k,–k) pairs of quasiparticles at the longitudinal polarization. This kind of absorption of microwaves occurs both in the ordered and specific spin-liquid phases, revealing the presence of quasiparticles in the specific spin-liquid phase.

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