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    Chiral orbital and spin textures, and Edelstein effects in monolayer Janus transition metal dichalcogenides

    Pratik Sahu1,2,*, S. Satpathy3,2,†, and B. R. K. Nanda1,2,‡

    • *Contact author: pratiksahu2413@gmail.com
    • †Contact author: satpathys@missouri.edu
    • ‡Contact author: nandab@iitm.ac.in

    Phys. Rev. B 113, 134435 – Published 21 April, 2026

    DOI: https://doi.org/10.1103/yccm-pwrz

    Abstract

    We investigate the orbital and spin Edelstein effect (OEE and SEE) in two-dimensional Janus transition metal dichalcogenides (TMDs) of the form MXX′ (M = Mo, W, Nb; X/X' = S, Se, Te) with the aid of density functional theory calculations and tight-binding model Hamiltonian studies. The chalcogen layers X and X′ break the mirror symmetry to introduce an internal electric field Eint normal to the plane, which is responsible for OEE and SEE. Our results show that in a non-Janus framework, the wave functions at the valence and conduction bands are dominated with the |x2−y2〉, |xy〉, and |z2〉 orbitals. Due to the Eint of the Janus system, these orbitals are now intermixed with the |xz〉 and |yz〉 orbitals to produce a robust orbital texture around the valleys Γ,K, and K′. The spin-orbit coupling, in addition to the formation of a spin texture, introduces a chirality reversal to the orbital texture. An applied in-plane electric field creates both OEE and SEE, which are comparable in magnitude. This makes the Janus materials promising for spin orbitronics. Our work paves the way for further experimental exploration for orbital and spin-orbital torque in Janus TMDs.

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