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    Phase diagrams of S=12 bilayer models of SU(2) symmetric antiferromagnets

    Fan Zhang1, Nisheeta Desai2, Wenan Guo1,3,*, and Ribhu K. Kaul4,†

    • *Contact author: waguo@bnu.edu.cn
    • †Contact author: ribhu.kaul@psu.edu

    Phys. Rev. B 113, 115120 – Published 10 March, 2026

    DOI: https://doi.org/10.1103/y58l-pcy1

    Abstract

    We study the T=0 phase diagrams of models of bilayers of S=1/2 square lattices antiferromagnets with SU(2) Heisenberg symmetry that have 2, 4, and 6 spin exchanges. We study two families of bilayer models with distinct internal symmetries and, hence, different phase diagram topologies. A traditional bilayer model in which the interlayer interaction is Heisenberg so that the two layers can exchange spin (and energy) with each other, making it possible to achieve a simple dimerized valence bond liquidlike state. The resulting phase diagram is rich with Néel, valence bond solid and simple dimer phases, and both first-order and continuous transitions, which we demonstrate are consistent with the conventional Landau theory of order parameters. In the second family of models in which the layers can exchange only energy but no spin (reminiscent of the Ashkin-Teller coupling), the simple dimer state cannot occur. The phase diagrams reveal a number of phase transitions that are accessed. We find that the phase transition between Néel and valence bond solid (VBS) is first order in both the spin-spin and energy-energy coupled models, although they have strikingly distinct finite-size scaling behavior and that the transition from VBS to dimer in the spin-spin coupling model deviates from the expected scenario of an XY model with dangerously irrelevant fourfold anisotropy.

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