Export citation

Export citation

Choose format for download:

Download Citation

    NMR evidence for an antisite-induced magnetic moment on Bi in the topological insulator heterostructure MnBi2Te4/(Bi2Te3)n

    R. Kalvig*, E. Jedryka, A. Lynnyk, P. Skupiński, K. Grasza, and M. Wójcik

    • *Contact author: kalvig@ifpan.edu.pl

    Phys. Rev. B 113, 184420 – Published 6 May, 2026

    DOI: https://doi.org/10.1103/y2t5-qbd7

    Abstract

    MnBi2Te4 (MBT) is the first intrinsic magnetic topological insulator, combining a topologically protected surface metallic state and intrinsic magnetic order. A structural compatibility with the nonmagnetic Bi2Te3 (BT) parent compound gives a possibility to create MBT/BT heterostructures and manipulate their magnetic state in view of optimizing the quantum anomalous Hall effect (QAHE). In this work an extensive nuclear magnetic resonance (NMR) study, supported by the bulk magnetization measurements, has been performed at 4.2 K on a self-organized single crystal MnBi2Te4/(Bi2Te3)n heterostructure, obtained from the Mn0.81Bi2.06Te4.13 melt. Mn55 and Bi209 NMR signals have been recorded as a function of the out-of-plane magnetic field up to 6 T, covering a spin-flop transition from the antiferromagnetic (AFM) to the canted antiferromagnetic configuration of the Mn layers. The canting angle at different external field values has been estimated based on NMR data. Presence of the AFM-coupled Mn antisites has been evidenced and shown to induce an antiparallel magnetic moment on Bi atoms within the host Bi layer. Detection of the induced magnetic moment on bismuth which contributes a new ferromagnetic component is of utmost importance for understanding the magnetic interactions in the MBT/BT system. These findings have potentially important implications for engineering the QAHE devices.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation