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  • Letter

Spin-polaron fingerprints in the optical conductivity of iridates

Francesco Cassol1,2,*, Léo Gaspard3,1, Cyril Martins3, Michele Casula1,†, and Benjamin Lenz1,‡

  • *Contact author: francesco.cassol@outlook.com
  • †Contact author: michele.casula@sorbonne-universite.fr
  • ‡Contact author: benjamin.lenz@sorbonne-universite.fr

Phys. Rev. B 113, L241107 – Published 2 June, 2026

DOI: https://doi.org/10.1103/xt5x-8c92

Abstract

As a consequence of their spin-orbit entangled ground state, many 5d5 iridate materials display a peculiar double-peak structure in optical transport quantities, such as absorption and conductivity. Their common interpretation is based on the presence of Hubbard subbands in the half-filled jeff=1/2 manifold. Herein, we challenge this picture, proposing a scenario based on the presence of spin-polaron (SP) quasiparticles, and assigning a dominant SP character to the first peak. We illustrate it by taking the materials Ba2IrO4 and Sr2IrO4 as paradigmatic examples, which we investigate within the dynamical mean-field theory and the self-consistent Born approximation. Both theories reproduce nontrivial features revealed by angle-resolved photoemission spectroscopy and optical transport measurements, supporting our interpretation. In the case of Sr2IrO4 we show how the SP scenario survives in the low-doped regime. Similar optical transport fingerprints are expected to be found in the wider class of 5d5 iridates and more generally in strongly correlated antiferromagnetic regimes, such as those found in cuprates.

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