Large-angle twisted bilayer graphene (TBLG) realizes a multicomponent quantum Hall (QH) platform of spin, valley, and layer pseudospins with strong Coulomb interaction-driven symmetry broken phases. Here, we investigate the low energy Landau-level spectrum of layer-decoupled TBLG and identify skyrmion-textured charged excitations and a field-induced insulating transition to an intervalley coherent state at zero-filling factor. Symmetric potential difference perpendicular to TBLG demonstrated layer coherent population of ground states with uniform energy barriers, while the charge imbalance in the layers at finite displacement field led to multidomain nucleation and a pronounced hysteresis in the exchange-dominated transport regime suggesting first order phase transitions between different QH ferromagnetic ground states.

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• Quantum Hall effect
• Quantum transport
• Twisted bilayer graphene