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    Quantum phase transition driven by competing intralayer and interlayer hopping in bilayer nickelates

    Xiaoyu Zhu1,*, Wei Qin2, Ping Cui1,3,†, and Zhenyu Zhang1,3

    • *Contact author: zxy00yxz@gmail.com
    • †Contact author: cuipg@ustc.edu.cn

    Phys. Rev. B 113, 075116 – Published 9 February, 2026

    DOI: https://doi.org/10.1103/xjpd-qlcr

    Abstract

    Bilayer nickelates exhibit high-temperature superconductivity under proper hydrostatic pressure or epitaxial strain, signifying the emergence of quantum phase transitions whose physical mechanisms remain unclear. Using a minimal bilayer Hubbard model incorporating only the Ni d3z2−r2 orbitals, we demonstrate that a phase transition naturally arises from tuning the ratio of intralayer to interlayer hopping amplitudes. The transition point separates regimes with a rich interplay between superconducting and density-wave orders. In the regime of weaker intralayer hopping, the ground state is characterized by quasi-long-range spin density wave order. As the intralayer hopping increases, the system undergoes a transition marked by the opening of a finite spin gap and the disappearance of spin density wave order. Meanwhile, superconductivity is dramatically enhanced, accompanied by the emergence of quasi-long-range charge density wave order, indicating that the system enters the Luther-Emery phase. This quantum phase transition, driven by the competition between intralayer and interlayer hopping, provides a plausible microscopic explanation for the experimentally observed correlation between the superconducting transition temperature and ratio of out-of-plane to in-plane lattice constants. Our findings reveal a possible link between the suppression of spin density wave order and the prominence of superconducting order, which may assist future efforts to optimize experimental conditions for further enhancing superconductivity in bilayer nickelates.

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