- Letter
Dynamic spin fluctuations in the = tetratrillium lattice antiferromagnet
Phys. Rev. B 114, L080403 – Published 11 August, 2026
DOI: https://doi.org/10.1103/xcr2-rxv6
Abstract
The three-dimensional (3D) magnet ( hosts an effective tetratrillium spin lattice of () ions, offering a prototypical platform to study frustration-driven phenomena in 3D. Through magnetization, specific heat, nuclear magnetic resonance (NMR), and muon spin relaxation () experiments, supported by first-principles calculations, we uncover an unconventional ground state. Despite strong antiferromagnetic interactions with a large Curie-Weiss temperature , no magnetic long-range order is observed down to 30 mK. Below , the NMR linewidth becomes nearly field independent and the spin-spin relaxation rate saturates, accompanied by a two-component relaxation in the transverse nuclear magnetization . The latter indicates the emergence of short-range dynamical correlations, which was further corroborated by a robust and field-insensitive broad maximum in specific heat. In , we detect neither a static internal field nor spin freezing; instead, the spins remain dynamic down to 30 mK and the asymmetry curves are best described by two coexisting dynamic relaxation channels: a dominant fast (sporadic) channel and a slower Markovian component. Their differing weights and fluctuation rates suggest microscopic inhomogeneity in spin dynamics. These persistent low-temperature spin fluctuations are found to be intrinsic to the 3D frustrated tetratrillium geometry, exemplifying (, a rare 3D antiferromagnet with a classical spin that fosters unconventional dynamics.