Export citation

Export citation

Choose format for download:

Download Citation
  • Letter

Dynamic spin fluctuations in the S = 52 tetratrillium lattice antiferromagnet KBaFe2(PO4)3

Sebin J. Sebastian1,2, Shams Sohel Islam3,*, R. Kolay1, S. Mohanty1, Q.-P. Ding2, Y. Skourski4, J. Sichelschmidt5, M. Baenitz5, Jonas A. Krieger3 et al.

T. J. Hicken3, H. Luetkens3, A. A. Tsirlin6, Y. Furukawa2,7,†, and R. Nath1,‡

  • *Contact author: shams.islam@psi.ch
  • †Contact author: furukawa@ameslab.gov
  • ‡Contact author: rameshchandra.nath@gmail.com

Phys. Rev. B 114, L080403 – Published 11 August, 2026

DOI: https://doi.org/10.1103/xcr2-rxv6

Abstract

The three-dimensional (3D) magnet KBaFe2(PO4)3 hosts an effective tetratrillium spin lattice of Fe3+ (S=5/2) ions, offering a prototypical platform to study frustration-driven phenomena in 3D. Through magnetization, specific heat, P31 nuclear magnetic resonance (NMR), and muon spin relaxation (µSR) experiments, supported by first-principles calculations, we uncover an unconventional ground state. Despite strong antiferromagnetic interactions with a large Curie-Weiss temperature θCW=−70(2)K, no magnetic long-range order is observed down to 30 mK. Below T*≃3.5K, the NMR linewidth becomes nearly field independent and the spin-spin relaxation rate 1/T2 saturates, accompanied by a two-component relaxation in the transverse nuclear magnetization Mxy. The latter indicates the emergence of short-range dynamical correlations, which was further corroborated by a robust and field-insensitive broad maximum in specific heat. In µSR, we detect neither a static internal field nor spin freezing; instead, the spins remain dynamic down to 30 mK and the asymmetry curves are best described by two coexisting dynamic relaxation channels: a dominant fast (sporadic) channel and a slower Markovian component. Their differing weights and fluctuation rates suggest microscopic inhomogeneity in spin dynamics. These persistent low-temperature spin fluctuations are found to be intrinsic to the 3D frustrated tetratrillium geometry, exemplifying KBaFe2(PO4)3, a rare 3D antiferromagnet with a classical spin that fosters unconventional dynamics.

Physics Subject Headings (PhySH)

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation