Export citation

Export citation

Choose format for download:

Download Citation

    Magnetotransport behavior and anomalous Hall effect of CVT grown single-crystalline topological Fe3−xGeTe2

    Rosni Roy, Sanat Kumar Adhikari, Riya Roy, Souvik Chatterjee, and Rajib Mondal*

    • *Contact author: mondal.rajib1988@gmail.com; rmondal@csr.res.in

    Phys. Rev. B 112, 054402 – Published 1 August, 2025

    DOI: https://doi.org/10.1103/x7dd-ngqk

    Abstract

    A detailed study of electrical transport, magnetotransport, anomalous, and topological Hall effect behavior of van der Waals force bonded layered single-crystalline Fe3−xGeTe2 (x≈0.3) have been performed. The single crystal of Fe3−xGeTe2, grown by the chemical vapor transport method, crystallizes in hexagonal crystal structure with space group P63/mmc. Temperature (T)-dependent dc magnetic susceptibility of Fe3−xGeTe2 depicts a paramagnetic to ferromagnetic transition at T≈180K (TC). Magnetic field variations of isothermal magnetization along the principal crystallographic directions in the magnetically ordered state at 5 K reveal soft ferromagnetic nature and significant magnetic anisotropy with the crystallographic c axis being the easy axis of magnetization. Temperature-dependent study of linear electrical resistivity reveals the metallic nature of Fe3−xGeTe2, exhibiting different scattering phenomena in three consecutive temperature regimes. The quadratic temperature dependence of linear electrical resistivity of Fe3−xGeTe2 below the magnetic ordering temperature gives a clear indication of the dominance of electron-magnon scattering. Magnetoresistance of Fe3−xGeTe2 along both the principal crystallographic directions are found to be negative and unsaturated with varying magnetic fields. The nature of the magnetic field dependence of magnetoresistance is very unusual, however exotic, revealing significant anisotropic behavior. Field-dependent magnetoresistance along the hard magnetization direction depicts quadratic magnetization dependence till the saturation magnetization field, which is reminiscent of the chiral spin texture of skyrmion host material. The study of Hall effect in Fe3−xGeTe2 depicts an anomalous Hall behavior, as expected. In addition, Hall effect of Fe3−xGeTe2 depicts a signature revealing nontrivial topological spin texture when magnetic field and current were applied along the basal ab plane, however perpendicular to each other. This type of topological Hall signature is expected for a candidate skyrmion host material like Fe3−xGeTe2.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation