Renormalized classical theory of quantum magnets
Phys. Rev. B 112, 134432 – Published 17 October, 2025
DOI: https://doi.org/10.1103/x7c2-x8p6
Abstract
We derive a renormalized classical spin (RCS) theory for quantum magnets by constraining a generalized classical theory that includes all multipolar fluctuations to a reduced phase space of dipolar SU(2) coherent states. When the spin Hamiltonian is linear in the spin operators for each lattice site , the RCS Hamiltonian coincides with the usual classical model . In the presence of nonlinear terms, however, the RCS theory is more accurate than . For the many materials modeled by spin Hamiltonians with (nonlinear) single-ion anisotropy terms, the use of the RCS theory is essential to accurately model phase diagrams and to extract the correct Hamiltonian parameters from neutron-scattering data.