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    Renormalized classical theory of quantum magnets

    David A. Dahlbom1,2, Hao Zhang1,3, Zoha Laraib1, Daniel M. Pajerowski2, Kipton Barros3, and Cristian D. Batista1,2

    Phys. Rev. B 112, 134432 – Published 17 October, 2025

    DOI: https://doi.org/10.1103/x7c2-x8p6

    Abstract

    We derive a renormalized classical spin (RCS) theory for S>1/2 quantum magnets by constraining a generalized classical theory that includes all multipolar fluctuations to a reduced CP1 phase space of dipolar SU(2) coherent states. When the spin Hamiltonian Ĥ(S) is linear in the spin operators Ŝj for each lattice site j, the RCS Hamiltonian H̃cl coincides with the usual classical model Hcl=limS→∞Ĥ(S). In the presence of nonlinear terms, however, the RCS theory is more accurate than Hcl. For the many materials modeled by spin Hamiltonians with (nonlinear) single-ion anisotropy terms, the use of the RCS theory is essential to accurately model phase diagrams and to extract the correct Hamiltonian parameters from neutron-scattering data.

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