Electronic correlations control interlayer coupling and magnetic transition in a heterostructure
Phys. Rev. B 112, 075406 – Published 7 August, 2025
DOI: https://doi.org/10.1103/x5cg-dxz6
Abstract
Bulk (MBT) is an intrinsic antiferromagnetic topological insulator. However, its low Néel temperature of K severely restricts its practical applications. Here, we propose a van der Waals heterostructure composed of monolayer MBT (ML-MBT) and monolayer , an intrinsic Chern insulator possessing a high Curie temperature (). By employing density functional theory calculations and Monte Carlo simulations, we demonstrate that interfacing ML-MBT with significantly enhances the of ML-MBT by a factor of four to five. Electronic correlations characterized by the Hubbard parameter for Mn- orbitals in play a crucial role in governing magnetic coupling within the system. At a moderate correlation strength of , slight structural distortions in break intralayer symmetry, enabling robust interlayer ferromagnetic coupling and yielding a single, unified magnetic transition. Increasing reduces these structural distortions, weakens interlayer coupling, and induces two distinct magnetic transitions, indicating interlayer magnetic decoupling. Thus, the heterostructure offers an interesting approach for controlling magnetic order and enhancing the performance of spintronic devices.