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    Electronic correlations control interlayer coupling and magnetic transition in a MnBi2Te4/MnBr3 heterostructure

    Yuanhao Zhu1,2, Xixi Yuan1, Ying Zhao1, Jin Zhang3, Zijing Ding2,*, and Huixia Fu1,4,†

    • *Contact author: zding@csrc.ac.cn
    • †Contact author: hxfu@cqu.edu.cn

    Phys. Rev. B 112, 075406 – Published 7 August, 2025

    DOI: https://doi.org/10.1103/x5cg-dxz6

    Abstract

    Bulk MnBi2Te4 (MBT) is an intrinsic antiferromagnetic topological insulator. However, its low Néel temperature of ∼25 K severely restricts its practical applications. Here, we propose a van der Waals heterostructure composed of monolayer MBT (ML-MBT) and monolayer MnBr3, an intrinsic Chern insulator possessing a high Curie temperature (TC∼200K). By employing density functional theory calculations and Monte Carlo simulations, we demonstrate that interfacing ML-MBT with MnBr3 significantly enhances the TC of ML-MBT by a factor of four to five. Electronic correlations characterized by the Hubbard parameter U2 for Mn-d orbitals in MnBr3 play a crucial role in governing magnetic coupling within the system. At a moderate correlation strength of U2=3.0eV, slight structural distortions in MnBr3 break intralayer symmetry, enabling robust interlayer ferromagnetic coupling and yielding a single, unified magnetic transition. Increasing U2 reduces these structural distortions, weakens interlayer coupling, and induces two distinct magnetic transitions, indicating interlayer magnetic decoupling. Thus, the MBT/MnBr3 heterostructure offers an interesting approach for controlling magnetic order and enhancing the performance of spintronic devices.

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