V and Se spectral reconstruction by charge density wave formation in probed by angle-resolved photoemission spectroscopy
Phys. Rev. B 113, 235112 – Published 5 June, 2026
DOI: https://doi.org/10.1103/wrhd-mksr
Abstract
The electronic structure of with charge density wave (CDW) transition has been studied by means of angle-resolved photoemission spectroscopy (ARPES) and scanning photoemission microscopy (SPEM). The partial depletion of the Fermi surfaces is observed in the CDW phase by ARPES, consistent with that reported previously. A flat band with V character, which is observed near the Fermi level around the point in the Brillouin zone, gains its spectral weight in the CDW phase while the holelike band around the point loses its weight. The spectral weight redistribution across the CDW transition indicates an important role of the V -Se hybridization, associated with the out-of-plane displacement of Se reported by Petkov et al. [Phys. Rev. B 111, 014105 (2025)]. The electronic inhomogeneity observed by SPEM suggests different surface terminations of the CDW state with the strong lattice and electronic modulation along the out-of-plane direction.