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Optical detection of four-spin chiral interaction in a two-dimensional honeycomb ferrimagnet

B. Murzaliev1, M. I. Katsnelson1,2, and M. Titov1

Phys. Rev. B 112, L100406 – Published 16 September, 2025

DOI: https://doi.org/10.1103/w7mp-rqgb

Abstract

The broken inversion symmetry of the magnetic lattice is normally described by Lifshitz invariants in a micromagnetic energy functional. Three exceptions are the lattices with Td, C3h, and D3h point group symmetries. For such lattices all Lifshitz invariants are forbidden despite broken inversion symmetry. In these cases the inversion symmetry breaking of the corresponding magnets is reflected by four-spin chiral invariants that are not related to the Dzyaloshinskii-Moriya interaction. The experimental detection of four-spin chiral interactions is an important task that has yet to be performed. We propose that the four-spin chiral interaction can be probed by energy-selective magnon relaxation in the two-dimensional ferromagnet Fe3GeTe2 that possesses D3h point group symmetry.

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