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    Emergence of a distinct density wave state in ultrathin VSe2 films

    Sen Liao1,*, Xiuhua Chen1,*, Yuzhe Wang1, Rui Xu1, Jianghao Yao1, Yilin Wang1,2,†, Donglai Feng2, and Juan Jiang1,2,‡

    • 1Hefei National Research Center for Physical Sciences at Microscale and School of Emerging Technology, University of Science and Technology of China, Hefei 230026, China
    • 2New Cornerstone Science Laboratory, Hefei National Laboratory, Hefei 230088, China

    • *These authors contributed equally to this work.
    • †Contact author: yilinwang@ustc.edu.cn
    • ‡Contact author: jjiangcindy@ustc.edu.cn

    Phys. Rev. B 113, 195142 – Published 21 May, 2026

    DOI: https://doi.org/10.1103/w4s8-fckc

    Abstract

    Dimensionality critically governs correlated states, often inducing emergent ground states in reduced dimensions. While VSe2 has been studied extensively, its monolayer ground state remains controversial. Here, we resolve these issues by investigating the thickness-dependent evolution of charge density waves (CDWs) and magnetism in VSe2. Using angle-resolved photoemission spectroscopy, we observe pronounced temperature-dependent band reconstruction uniquely emerging in bilayer and monolayer VSe2, in sharp contrast to bulk and multilayer VSe2. While a 3×7 CDW accounts for the reconstructed band topology, it fails to explain the global suppression of spectral weight at low temperature. Instead, DFT calculations suggest that a coupled 3×7 spin density wave (SDW)+CDW state can quantitatively account for all key experimental observations. These results are consistent with a thickness-driven crossover to a coupled SDW+CDW state, establishing VSe2 as a tunable platform for exploring intertwined spin-charge orders in two-dimensional quantum materials.

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