Emergence of a distinct density wave state in ultrathin films
Phys. Rev. B 113, 195142 – Published 21 May, 2026
DOI: https://doi.org/10.1103/w4s8-fckc
Abstract
Dimensionality critically governs correlated states, often inducing emergent ground states in reduced dimensions. While has been studied extensively, its monolayer ground state remains controversial. Here, we resolve these issues by investigating the thickness-dependent evolution of charge density waves (CDWs) and magnetism in . Using angle-resolved photoemission spectroscopy, we observe pronounced temperature-dependent band reconstruction uniquely emerging in bilayer and monolayer , in sharp contrast to bulk and multilayer . While a CDW accounts for the reconstructed band topology, it fails to explain the global suppression of spectral weight at low temperature. Instead, DFT calculations suggest that a coupled spin density wave state can quantitatively account for all key experimental observations. These results are consistent with a thickness-driven crossover to a coupled state, establishing as a tunable platform for exploring intertwined spin-charge orders in two-dimensional quantum materials.
Physics Subject Headings (PhySH)
- Antiferromagnetism
- Band gap
- Charge density waves
- Electronic structure
- Magnetic phase transitions
- Magnetism
- Nesting
- Phase diagrams
- Phase transitions
- 2-dimensional systems
- Antiferromagnets
- Magnetic thin films
- Transition metal dichalcogenides
- Ultrathin films
- Angle-resolved photoemission spectroscopy
- Density functional theory
- First-principles calculations
- Methods in magnetism
- Molecular beam epitaxy