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    Fermi-liquid behavior and characteristic temperature-dependent susceptibility in clean single crystal RuO2

    Shubhankar Paul1,2,3, Atsutoshi Ikeda2, Hisakazu Matsuki1,4, Giordano Mattoni1, Jörg Schmalian5, Kunihiko Yamauchi6, Chanchal Sow3, Shingo Yonezawa2, and Yoshiteru Maeno1,7

    Phys. Rev. B 114, 034414 – Published 10 July, 2026

    DOI: https://doi.org/10.1103/vy8x-q3l6

    Abstract

    The magnetic nature of the altermagnet candidate RuO2 remains under debate. It has been recently shown from quantum oscillations and angle-resolved photoemission spectroscopy that the high-quality RuO2 bulk single crystal is a paramagnetic metal. Here we report the specific heat and magnetic susceptibility in ultraclean RuO2 single crystals with residual resistivity ratio up to 1200. The electronic specific heat, the magnetic susceptibility, and the T2 coefficient in resistivity point to a weakly correlated three-dimensional Fermi-liquid state, as supported by the Wilson and Kadowaki-Woods ratios. The magnetic susceptibility increases with temperature and is phenomenologically fitted with an inclusion of Tln(T/T0) over a wide temperature range up to 400 K. In contrast, the energy dependence of the density of states and thermal activation of quasiparticles lead to a decrease with temperature. Such characteristic temperature dependence, similar to that observed in other d-electron metals, is attributable to an enhanced orbital contribution arising from lattice-expansion-induced changes in the band structure.

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