High-frequency magnetotransport in samples synthesized by microwave irradiation versus conventional heating
Phys. Rev. B 114, 274402 – Published 2 November, 2026
DOI: https://doi.org/10.1103/vvyg-lqh6
Abstract
Magnetoresistance of hole-doped at frequencies above a few MHz has been seldom reported compared to numerous studies on magnetoresistance measured at direct current. Here, we contrast the high-frequency magnetoresistance in the frequency range in polycrystalline (LMO) synthesized by microwave irradiation of oxide precursors in a microwave furnace (MW-LMO) and by conventional heating (CH-LMO) in an electrical furnace. The structure at room temperature changes from orthorhombic in CH-LMO to rhombohedral in MW-LMO. A combination of magnetization and resistivity studies suggests that the CH-LMO sample is a canted antiferromagnetic insulator below 140 K but the MW-LMO is a ferromagnetic metal with . While the high-frequency resistance of the CH-LMO sample at 300 K decreases gradually with increasing strength of the applied dc magnetic field for all , a peak appears at when in the MW-LMO sample and increases linearly with . We attribute the observed features in the high-frequency magnetoresistance of MW-LMO to current-driven resonant excitation of spins in the paramagnetic state. Its absence in the CH-LMO sample highlights the need for an optimum hole density to observe this effect.