Type-III Weyl semi-half-metal in an ultralight monolayer
Phys. Rev. B 112, 195126 – Published 20 November, 2025
DOI: https://doi.org/10.1103/vqdz-12bz
Abstract
The interplay between magnetic ordering and band topology has emerged as a fertile ground for discovering novel quantum states with profound implications for fundamental physics and next-generation electronics. Here, we theoretically predict a different type-III Weyl semi-half-metal (SHM) state in monolayer , uniquely combining magnetic half-metallicity and type-III Weyl semimetal characteristics. First-principles calculations reveal a fully spin polarized and critically tilted Weyl cone around the Fermi level in monolayer , driven by -orbital ferromagnetism. This arises from the symmetry-protected band crossing between a partially flat valence band and a highly dispersive conduction band, leading to type-III Weyl fermions with strong transport anisotropy. A low-energy Hamiltonian is constructed and corresponding nontrivial edge states are uncovered to capture the topological nature of . Notably, this Weyl SHM phase remains robust under biaxial strain ranging from to , with an ideal type-III Weyl fermion emerging alongside a linelike ergodic surface emerging at strain, offering a promising platform for exploring correlated electronic phenomena. Our results establish as a viable candidate for realizing exotic type-III Weyl SHM states and open an avenue for exploring the intricate interplay among magnetism, topology, and flat-band physics.