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Pressure-induced reentrant superconductivity in the misfit layered compound (SnS)1.15(TaS2)

Chutong Zhang1,2,*, Jiajia Feng3,*, Xiao Tang1,2,*, Xiangzhuo Xing1,2,†, Na Zuo1,2, Xiaolei Yi4, Yan Meng5, Xiaoran Zhang1,2,‡, Rajesh Kumar Ulaganathan6 et al.

Raman Sankar7, Xiaofeng Xu8, Xin Chen1,2,§, and Xiaobing Liu1,2

  • *These authors contributed equally to this work.
  • †Contact author: xzxing@qfnu.edu.cn
  • ‡Contact author: xiaoran_zhang@qfnu.edu.cn
  • §Contact author: chenxin@qfnu.edu.cn

Phys. Rev. B 113, L140506 – Published 29 April, 2026

DOI: https://doi.org/10.1103/vcqm-h54l

Abstract

Misfit layered compounds are natural van der Waals heterostructures in which electronically active transition-metal dichalcogenide layers are decoupled by incommensurate blocking layers, enabling bulk realization of quasi-two-dimensional quantum states. Here we investigate the superconducting, transport, and structural properties of the misfit compound (SnS)1.15(TaS2) under pressures up to ∼150 GPa. The low-pressure superconducting phase is gradually suppressed and disappears near 14.7 GPa. Remarkably, a distinct superconducting phase reemerges above ∼80 GPa and persists to the highest pressures achieved. This reentrant superconductivity follows a pressure-induced sign reversal of the Hall coefficient near 60 GPa and a nonmonotonic evolution of the normal-state resistance, indicating an intimate connection with pressure-driven electronic reconstruction. Our work demonstrates a pressure-driven electronic reconstruction leading to reentrant superconductivity in a misfit layered compound, establishing pressure as an effective route to engineer superconductivity and electronic states in natural van der Waals heterostructures.

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