Export citation

Export citation

Choose format for download:

Download Citation

    Multimagnon and multispinon L3-edge RIXS spectra of an effective J̃1−J̃2−J̃3 square-lattice Heisenberg model

    Kai-Yuan Qi (祁开元)1, Shangjian Jin1, Trinanjan Datta2,*, and Dao-Xin Yao (姚道新)1,†

    • 1State Key Laboratory of Optoelectronic Materials and Technologies, Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, Center for Neutron Science and Technology, School of Physics, Sun Yat-Sen University, Guangzhou 510275, China
    • 2Department of Physics and Biophysics, Augusta University, 1120 15th Street, Augusta, Georgia 30912, USA

    • *Contact author: tdatta@augusta.edu
    • †Contact author: yaodaox@mail.sysu.edu.cn

    Phys. Rev. B 112, 134438 – Published 23 October, 2025

    DOI: https://doi.org/10.1103/vc7b-15sf

    Abstract

    We investigate the multimagnon and the multispinon L3-edge resonant inelastic x-ray scattering (RIXS) spectra of a spin-1/2 effective J̃1−J̃2−J̃3 square lattice Heisenberg model in its Néel ordered phase. Motivated by the observation of satellite intensity peaks above the single magnon dispersion in the L-edge RIXS spectrum, we propose a resonating valence bond (RVB) inspired RIXS mechanism that incorporates the local site ultrashort core-hole lifetime (UCL) expansion. We compute the multimagnon and the multispinon excitations using O(1/S) interacting spin-wave theory and Schwinger boson mean-field theory (SBMFT) formalism, respectively. We treat the x-ray scattering process up to second order in the UCL expansion. Our calculations of two-magnon, bimagnon, and three-magnon RIXS intensities reveal that interacting spin-wave theory fails to fully capture all the quantum correlations in the antiferromagnetic ordered phase. However utilizing the SBMFT framework, with a ground state that incorporates features of both the Néel order and fluctuating RVB components, we demonstrate that a RIXS bond-flipping mechanism provides an alternative deeper physical explanation of the satellite intensities. Specifically, we find that the spin-correlation spectra predicted by the fluctuating RVB mechanism aligns with higher-order UCL expansion results. We further show that the satellite intensity above the single-magnon mode can originate both from a one-to-three-magnon hybridization vertex process and from condensed spinons exhibiting Higgs mechanism. These features reflect the interplay of quantum fluctuation, entanglement, and gauge interaction effects of quantum magnetism probed by RIXS.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    Supplemental Material (Subscription Required)

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation