Export citation

Export citation

Choose format for download:

Download Citation

    Decisive role of an extra Fe sublattice: Frustration, criticality, and skyrmions in the van der Waals ferromagnets Fe5GeTe2 versus Fe3GeTe2

    Jyoti Saini1, Ankita Tiwari1,2, Pawan Kumar Srivastava3,4, Changgu Lee3,5, and Subhasis Ghosh1,*

    • *Contact author: subhasis.ghosh.jnu@gmail.com

    Phys. Rev. B 113, 214451 – Published 23 June, 2026

    DOI: https://doi.org/10.1103/v9rm-l6vb

    Abstract

        The van der Waals magnets Fe3GeTe2 and Fe5GeTe2, chemically similar yet magnetically distinct, provide an ideal platform for probing how structural complexity governs emergent magnetic order, anisotropy, and topological textures. Fe3GeTe2 does not host skyrmions, whereas Fe5GeTe2 does, raising fundamental questions about the roles of inversion symmetry, frustration, and exchange interactions. Through comprehensive magnetization, susceptibility, and critical exponent analysis, we demonstrate that magnetic frustration, absent in Fe3GeTe2, is crucial in Fe5GeTe2. The extra Fe+ sublattice in Fe5GeTe2 breaks inversion symmetry, introduces competing exchange, and yields a significant frustration parameter f≈ 3.8. Critical exponent analysis reveals field-driven crossover from a mean field to a 2D-Heisenberg class with increasing field in Fe3GeTe2, whereas field-driven crossover from a frustrated 3D-Heisenberg class (β=0.348,γ=1.32) at low fields reveals a conventional 3D-Heisenberg class (β=0.368,γ=1.368) at high fields in Fe5GeTe2. Our results establish magnetic frustration, rather than the Dzyaloshinskii-Moriya interaction alone, as the key ingredient stabilizing skyrmionic phases, offering a design principle for topological spin textures in layered van der Waals magnets. We show here that an extra sublattice in Fe5GeTe2 is essentially responsible for most of the differences in magnetic properties between Fe3GeTe2 and Fe5GeTe2.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    Supplemental Material (Subscription Required)

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation