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    Magnetic dilution in the triangular lattice antiferromagnet NaYb1−xLuxO2

    Steven J. Gomez Alvarado1, Brenden R. Ortiz2, Soren Bear1, Benito A. Gonzalez1, Andrea N. Capa Salinas1, Adam Berlie3, Michael J. Graf4, and Stephen D. Wilson1,*

    • *Contact author: stephendwilson@ucsb.edu

    Phys. Rev. B 112, 144434 – Published 21 October, 2025

    DOI: https://doi.org/10.1103/th1p-5rxt

    Abstract

    The delafossitelike compound NaYbO2 hosts a triangular lattice of Yb3+ moments and is a promising candidate for the realization of a quantum spin liquid ground state—an exotic, quantum-disordered magnetic phase featuring long-range entanglement of spins. Tuning this system away from this quantum-disordered regime toward classical order or spin freezing is a powerful approach to shed light on the nature of the parent ground state. Here we leverage the substitution of nonmagnetic Lu3+ onto the Yb3+ sites to study the effects of magnetic disorder in NaYbO2 using low-temperature ac susceptibility, heat capacity, and muon spin relaxation (μSR) measurements. Our μSR measurements reveal resilient, correlated magnetic fluctuations that persist to at least 15% dilution, precluding conventional spin freezing and magnetic inhomogeneity. Heat capacity and magnetic susceptibility resolve a rapid suppression of the field-induced “up-up-down” magnetic order upon dilution and a crossover in the power-law behavior of the low-temperature magnetic excitations associated with the zero-field quantum disordered ground state. Taken together, these results support the notion of a robust network of entangled moments in NaYbO2 and provide experimental validation of several models of a Heisenberg triangular lattice antiferromagnet in the presence of disorder.

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