Fragile long-range antiferromagnetic order in the triangular-lattice quantum magnet
Phys. Rev. B 113, 214422 – Published 5 June, 2026
DOI: https://doi.org/10.1103/tf6x-rht3
Abstract
Rare-earth triangular lattices provide an ideal platform for exploring novel quantum magnetic states. Here, we report the crystal growth and magnetic properties of a rare-earth triangular-lattice compound, . Alternating-current magnetic susceptibility and specific heat measurements reveal a long-range antiferromagnetic order below . The long-range magnetic order can be rapidly suppressed by a small magnetic field of along the axis, followed by a broad field-induced anomaly above 0.05 T that shifts to higher temperatures as the magnetic field increases. The magnetic entropy release below 2 K is estimated to be , which is consistent with a Kramers doublet described by an effective spin . Finally, a magnetic field-temperature contour map is constructed based on the specific heat results. Our work identifies a long-range yet fragile magnetic order in this newly grown quantum magnet, and its fragility suggests the presence of strong quantum fluctuations arising from geometric frustrations and quantum spins in .