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    Fragile long-range antiferromagnetic order in the triangular-lattice quantum magnet ErZn3P3

    Yimin Wang, Peiyue Ma, Weijie Lin, Ye Xia, Yujie Wang, Ruixiang Jiang, Xinlei Liu, Chaoxin Huang, Tao Xie* et al.

    Meng Wang†

    • Institute of Neutron Science and Technology, Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-sen University, Guangzhou 510275, China

    • *Contact author: xiet69@mail.sysu.edu.cn
    • †Contact author: wangmeng5@mail.sysu.edu.cn

    Phys. Rev. B 113, 214422 – Published 5 June, 2026

    DOI: https://doi.org/10.1103/tf6x-rht3

    Abstract

    Rare-earth triangular lattices provide an ideal platform for exploring novel quantum magnetic states. Here, we report the crystal growth and magnetic properties of a rare-earth triangular-lattice compound, ErZn3P3. Alternating-current magnetic susceptibility and specific heat measurements reveal a long-range antiferromagnetic order below T=0.12K. The long-range magnetic order can be rapidly suppressed by a small magnetic field of μ0H=0.04T along the c axis, followed by a broad field-induced anomaly above 0.05 T that shifts to higher temperatures as the magnetic field increases. The magnetic entropy release below 2 K is estimated to be 0.852(42)Rln2, which is consistent with a Kramers doublet described by an effective spin S=1/2. Finally, a magnetic field-temperature contour map is constructed based on the specific heat results. Our work identifies a long-range yet fragile magnetic order in this newly grown S=1/2 quantum magnet, and its fragility suggests the presence of strong quantum fluctuations arising from geometric frustrations and quantum spins in ErZn3P3.

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