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Dominance of the orbital Hall effect over spin in transition metal heterostructures

J. L. Costa1,*, E. Santos1, J. B. S. Mendes2, and A. Azevedo1,†

  • *Contact author: jefferson.limacosta@ufpe.br
  • †Contact author: antonio.azevedo@ufpe.br

Phys. Rev. B 112, 054443 – Published 20 August, 2025

DOI: https://doi.org/10.1103/tbdz-jc6k

Abstract

We study inverse spin and orbital Hall effects in 19 transition metals using spin pumping driven by ferromagnetic resonance. Spin-to-charge conversion was measured in YIG/X(5), while orbital-to-charge conversion was probed in YIG/Pt(2)/X(5) heterostructures. Here, X represents the different transition metals. We observe that even metals with relatively weak spin-orbit coupling can exhibit strong orbital-to-charge conversion. Surprisingly, the orbital contribution overwhelmingly dominates over the spin response, clarifying the challenge of disentangling these effects. Our results largely agree with first-principles predictions for spin and orbital Hall conductivities but reveal discrepancies in select materials.

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