Export citation

Export citation

Choose format for download:

Download Citation

    Enhanced superconductivity in two-dimensional Cu2N: First-principles investigation of electron-phonon coupling and topological properties

    Guang-ren Na, Meng-hui Wang, and Rui Bian

    Zhong-hua Cui*

    • Institute of Atomic and Molecular Physics, Jilin University, Changchun 130023, China

    • *Contact author: zcui@jlu.edu.cn

    Phys. Rev. B 112, 224504 – Published 2 December, 2025

    DOI: https://doi.org/10.1103/t7nc-p31n

    Abstract

    Two-dimensional materials with intrinsic superconductivity and nontrivial topology represent a frontier for discovering exotic quantum states and potential applications in quantum devices. Here, we report the first comprehensive theoretical investigation of superconductivity in monolayer and bilayer Cu2N. The monolayer Cu2N has been recently synthesized experimentally and features a unique checkerboard lattice with topological nodal lines. Following this experimental breakthrough, we predict phonon-mediated superconductivity with transition temperatures (Tc) of 3.8 K (monolayer) and 7.9 K (bilayer) arising from strong electron-phonon coupling (λ=0.76 and 0.84, respectively) mediated primarily by Cu d-orbitals and low-frequency phonon modes. The bilayer shows 84% Tc enhancement through additional interlayer vibrational modes that strengthen Cu d-orbital coupling via enhanced out-of-plane vibrations. Strain engineering enhances monolayer Tc to 4.5 K under 0.2% compressive strain through optimized electronic density of states and phonon softening. We identify a practical synthesis pathway involving multilayer growth followed by controlled exfoliation with moderate energy cost (0.97J/m2). Our results demonstrate that Cu2N, featuring coexisting topological nodal lines and phonon-mediated superconductivity, represents a promising experimental platform for investigating potential topological superconducting behavior in accessible two-dimensional systems.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    Supplemental Material (Subscription Required)

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation