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Resolving exciton and polariton multiparticle correlations in an optical microcavity in the strong-coupling regime

Victoria Quirós-Cordero1,*, Esteban Rojas-Gatjens2,3,*, Martin Gomez-Dominguez1, Hao Li4, Carlo A. R. Perini1, Natalie Stingelin1,5, Juan-Pablo Correa-Baena1, Eric R. Bittner6, Ajay Ram Srimath Kandada7,† et al.

Carlos Silva-Acuña2,4,‡

  • *These authors equally contributed to this work.
  • †Contact author: srimatar@wfu.edu
  • ‡Contact author: carlos.silva@umontreal.ca

Phys. Rev. B 113, L041102 – Published 2 January, 2026

DOI: https://doi.org/10.1103/t2b9-3vby

Abstract

Multiparticle correlations of exciton polaritons and reservoir excitons in the strong light-matter coupling regime dictate the quantum dynamics of optical microcavities. In this work, we examine the many-body exciton-polariton dynamics in a Fabry-Pérot microcavity of a two-dimensional metal-halide semiconductor over timescales involving polariton (≪1ps) and exciton (≫1ps) scattering. We find enhanced exciton nonlinear dynamics in the microcavity versus the bare semiconductor, concomitant with ultrafast polariton scattering dynamics. We measure, by means of coherent spectroscopy, the coupling between exciton polaritons, bright excitons, and reservoir excitons that highlight the complex scattering landscape that fundamentally drives polariton condensation.

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