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Thermodynamics and heat transport of a Yb3Sc2Ga3O12 single crystal: A quantum spin liquid candidate

Y. F. Xin1,*, A. Rutherford2,*, N. Li1,†, M. L. Feng1, Y. J. Liu1, Z. Y. Zhao1, Y. Y. Wang1, H. Liang1, Y. Zhou1 et al.

Q. J. Li3, M. Y. Xu4, W. Xie4, E. S. Choi5, X. Zhao6, J. Ma7, H. D. Zhou2,‡, and X. F. Sun1,§

  • 1Anhui Provincial Key Laboratory of Magnetic Functional Materials and Devices, Institutes of Physical Science and Information Technology, Anhui University, Hefei, Anhui 230601, People's Republic of China
  • 2Department of Physics and Astronomy, University of Tennessee, Knoxville, Tennessee 37996, USA
  • 3School of Physics and Optoelectronics, Anhui University, Hefei, Anhui 230061, People's Republic of China
  • 4Department of Chemistry, Michigan State University, East Lansing, Michigan 48824, USA
  • 5National High Magnetic Field Laboratory, Florida State University, Tallahassee, Florida 32310-3706, USA
  • 6School of Physical Sciences, University of Science and Technology of China, Hefei, Anhui 230026, People's Republic of China
  • 7Key Laboratory of Artificial Structures and Quantum Control, Shenyang National Laboratory for Materials Science, School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China

  • *These authors contributed equally to this work.
  • †Contact author: nli@ahu.edu.cn
  • ‡Contact author: hzhou10@utk.edu
  • §Contact author: xfsun@ahu.edu.cn

Phys. Rev. B 113, 014436 – Published 27 January, 2026

DOI: https://doi.org/10.1103/styt-544l

Abstract

High-quality single crystals of Yb3Sc2Ga3O12 with a hyperkagome spin lattice were grown by using the floating-zone method. The magnetic susceptibility, specific heat and thermal conductivity were measured down to very low temperatures (<100 mK) to characterize the magnetic properties and probe the nature of ground state. The experimental results demonstrate that the ground state is spin disordered one with effective 1/2 spin and antiferromagnetic coupling, pointing to a possible quantum spin liquid, although the clear characteristic behaviors of quantum spin liquid were not observed in these results. The specific heat data display broad peaklike feature that is likely caused by the short-range spin correlations. The ultralow-temperature thermal conductivity exhibits rather strong magnetic field dependence and zero residual term (κ0/T), which indicates the scattering between phonons and magnetic excitations. In addition, both the specific heat and thermal conductivity data display some field-induced magnetic transitions.

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