Spin canting and ordered moments driven by tetragonal compression in ruthenates
Phys. Rev. B 113, 054433 – Published 20 February, 2026
DOI: https://doi.org/10.1103/stt1-v24p
Abstract
Spin-orbit coupling in transition-metal oxides entangles lattice, charge, and spin degrees of freedom to generate unconventional magnetic states. In Sn-doped , compression of the octahedra enhances the -ordered moment and drives -axis spin canting via Dzyaloshinskii-Moriya interactions from staggered octahedral tilts and rotations. Neutron diffraction, depolarization, and magnetization measurements reveal a canted component () together with a weak ferromagnetic response. These results demonstrate that tetragonal compression stabilizes an in-plane canted AFM state with enhanced moment, establishing it as an effective lever to engineer spin-orbit entangled magnetism in layered ruthenates.