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Phonon scattering mechanisms in WTe2 observed by ultrafast coherent phonon spectroscopy

Mizuki Akei*, Yu Mizukoshi, and Muneaki Hase†

  • Department of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba, 1-1-1 Tennodai, Tsukuba 305-8573, Japan

  • *Contact author: s2630089@u.tsukuba.ac.jp
  • †Contact author: mhase@bk.tsukuba.ac.jp

Phys. Rev. B 114, L080303 – Published 5 August, 2026

DOI: https://doi.org/10.1103/ssvg-wh36

Abstract

Revealing the mechanisms of phonon scattering is crucial for understanding material properties such as transport characteristics and optical responses. It can be discussed by measuring the temperature dependence of the phonon energy and lifetime. To gain insight into these mechanisms in the Weyl semimetal Td−WTe2, we investigated coherent phonons using time-resolved pump-probe spectroscopy in a wide temperature range from 4.6 to 300 K. The temperature dependence of the frequency and decay rate of the two high-frequency optical modes was described by the conventional anharmonic phonon-phonon scattering model. In contrast, the low-frequency mode at 2.4 THz exhibited anomalous behavior, which can be interpreted as the contribution of phonon-electron scattering.

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