Stacking-controlled altermagnetism and Rashba splitting in bilayer
Phys. Rev. B 113, 184448 – Published 26 May, 2026
DOI: https://doi.org/10.1103/sjgg-yn11
Abstract
Altermagnetism is a recently identified magnetic phase characterized by symmetry-enforced nonrelativistic spin splitting despite vanishing net magnetization. Here, using spin-space symmetry analysis and first-principles calculations, we show that inversion-symmetry-broken stackings of bilayer , a two-dimensional van der Waals antiferromagnet with localized Gd moments, host stacking-tunable altermagnetism. While the magnetic order originates from localized electrons, the altermagnetic spin splitting is carried by I states near the Fermi level, revealing a separation between the source of magnetism and the electronic states that encode the spin texture. Specific stackings, namely, and , realize symmetry-protected altermagnetic phases, whereas the stacking remains spin degenerate. Moreover, the stackings simultaneously develop out-of-plane ferroelectric polarization, while the stackings remain nonferroelectric due to cancellation of local dipoles. Upon including spin-orbit coupling, the relevant antiunitary symmetries are lifted and the system transitions from an altermagnetic regime to a Rashba-type spin-split state with a rich momentum-space spin texture, while the total magnetization remains nearly zero. Our results establish bilayer as a stacking-tunable platform for exploring the symmetry connection between altermagnetism, ferroelectricity, and relativistic spin textures.