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    Stacking-controlled altermagnetism and Rashba splitting in bilayer GdI3

    Yaxin Pan, Yihang Bai, Fengzhu Ren, Bing Wang*, and Jun-Hyung Cho†

    • Joint Center for Theoretical Physics, Institute for Computational Materials Science, Henan Key Laboratory of High Efficiency Energy Conversion Science and Technology, and Henan International Joint Laboratory of New Energy Materials and Devices, School of Physics and Electronics, Henan University, Kaifeng 475004, China

    • *Contact author: wb@henu.edu.cn
    • †Contact author: cho@henu.edu.cn

    Phys. Rev. B 113, 184448 – Published 26 May, 2026

    DOI: https://doi.org/10.1103/sjgg-yn11

    Abstract

    Altermagnetism is a recently identified magnetic phase characterized by symmetry-enforced nonrelativistic spin splitting despite vanishing net magnetization. Here, using spin-space symmetry analysis and first-principles calculations, we show that inversion-symmetry-broken stackings of bilayer GdI3, a two-dimensional van der Waals antiferromagnet with localized Gd 4f moments, host stacking-tunable altermagnetism. While the magnetic order originates from localized 4f electrons, the altermagnetic spin splitting is carried by I p states near the Fermi level, revealing a separation between the source of magnetism and the electronic states that encode the spin texture. Specific stackings, namely, AB*/BA* and AC*/CA*, realize symmetry-protected altermagnetic phases, whereas the AA* stacking remains spin degenerate. Moreover, the AB*/BA* stackings simultaneously develop out-of-plane ferroelectric polarization, while the AC*/CA* stackings remain nonferroelectric due to cancellation of local dipoles. Upon including spin-orbit coupling, the relevant antiunitary symmetries are lifted and the system transitions from an altermagnetic regime to a Rashba-type spin-split state with a rich momentum-space spin texture, while the total magnetization remains nearly zero. Our results establish bilayer GdI3 as a stacking-tunable platform for exploring the symmetry connection between altermagnetism, ferroelectricity, and relativistic spin textures.

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