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Three-dimensional topological orbital Hall effect caused by magnetic hopfions
Phys. Rev. B 112, 134426 – Published 15 October, 2025
DOI: https://doi.org/10.1103/sc9g-l9by
Abstract
Magnetic hopfions are noncollinear spin textures that are characterized by an integer topological invariant, called the Hopf index. The three-dimensional magnetic solitons can be thought of as a tube with a twisted magnetization that has been closed at both ends to form a torus. The tube consists of a magnetic whirl called an in-plane skyrmion or bimeron. Although hopfions have been observed by microscopy techniques, their detection remains challenging as they lack an electronic hallmark so far. Here we predict a three-dimensional orbital Hall effect caused by hopfion textures: When an electric field is applied, the hopfion generates a transverse current of orbital angular momentum. The effect arises due to the local emergent field that gives rise to in-plane and out-of-plane orbital Hall conductivities. This orbital Hall response can be seen as a hallmark of hopfions and allows us to distinguish them from other textures, such as skyrmioniums, that look similar in real-space microscopy experiments. While the two-dimensional topological invariant of a skyrmion determines its topological Hall transport, the unique three-dimensional topological orbital Hall effect can be identified with the three-dimensional topological invariant that is the Hopf index. Our results make hopfions attractive for spin-orbitronic applications because their orbital signatures allow for their detection in devices and give rise to large orbital torques.
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References (98)
- B. Göbel, I. Mertig, and O. A. Tretiakov, Beyond skyrmions: Review and perspectives of alternative magnetic quasiparticles, Phys. Rep. 895, 1 (2021).
- A. N. Bogdanov and D. A. Yablonskii, Thermodynamically stable “vortices” in magnetically ordered crystals. The mixed state of magnets, Zh. Eksp. Teor. Fiz. 95, 178 (1989) [Sov. Phys. JETP 68, 101 (1989)].
- S. Mülbauer, B. Binz, F. Jonietz, C. Pfleiderer, A. Rosch, A. Neubauer, R. Georgii, and P. Böni, Skyrmion lattice in a chiral magnet, Science 323, 915 (2009).
- X. Yu, Y. Onose, N. Kanazawa, J. Park, J. Han, Y. Matsui, N. Nagaosa, and Y. Tokura, Real-space observation of a two-dimensional skyrmion crystal, Nature (London) 465, 901 (2010).
- N. Nagaosa, J. Sinova, S. Onoda, A. H. MacDonald, and N. P. Ong, Anomalous Hall effect, Rev. Mod. Phys. 82, 1539 (2010).
- A. K. Nayak, V. Kumar, T. Ma, P. Werner, E. Pippel, R. Sahoo, F. Damay, U. K. Rößler, C. Felser, and S. S. Parkin, Magnetic antiskyrmions above room temperature in tetragonal Heusler materials, Nature (London) 548, 561 (2017).
- L. Peng, R. Takagi, W. Koshibae, K. Shibata, K. Nakajima, T.-h. Arima, N. Nagaosa, S. Seki, X. Yu, and Y. Tokura, Controlled transformation of skyrmions and antiskyrmions in a non-centrosymmetric magnet, Nat. Nanotechnol. 15, 181 (2020).
- J. Jena, B. Göbel, T. Ma, V. Kumar, R. Saha, I. Mertig, C. Felser, and S. S. Parkin, Elliptical Bloch skyrmion chiral twins in an antiskyrmion system, Nat. Commun. 11, 1115 (2020).
- Y. A. Kharkov, O. P. Sushkov, and M. Mostovoy, Bound states of skyrmions and merons near the Lifshitz point, Phys. Rev. Lett. 119, 207201 (2017).
- B. Göbel, A. Mook, J. Henk, I. Mertig, and O. A. Tretiakov, Magnetic bimerons as skyrmion analogues in in-plane magnets, Phys. Rev. B 99, 060407(R) (2019).
- N. Gao, S.-G. Je, M.-Y. Im, J. W. Choi, M. Yang, Q.-C. Li, T. Wang, S. Lee, H.-S. Han, K.-S. Lee et al., Creation and annihilation of topological meron pairs in in-plane magnetized films, Nat. Commun. 10, 5603 (2019).
- N. Nagaosa and Y. Tokura, Topological properties and dynamics of magnetic skyrmions, Nat. Nanotechnol. 8, 899 (2013).
- P. Bruno, V. K. Dugaev, and M. Taillefumier, Topological Hall effect and Berry phase in magnetic nanostructures, Phys. Rev. Lett. 93, 096806 (2004).
- A. Neubauer, C. Pfleiderer, B. Binz, A. Rosch, R. Ritz, P. Niklowitz, and P. Böni, Topological Hall effect in the A phase of MnSi, Phys. Rev. Lett. 102, 186602 (2009).
- M. Lee, W. Kang, Y. Onose, Y. Tokura, and N. P. Ong, Unusual Hall effect anomaly in MnSi under pressure, Phys. Rev. Lett. 102, 186601 (2009).
- M. Raju, A. Petrović, A. Yagil, K. Denisov, N. Duong, B. Göbel, E. Şaşıoğlu, O. Auslaender, I. Mertig, I. Rozhansky et al., Colossal topological Hall effect at the transition between isolated and lattice-phase interfacial skyrmions, Nat. Commun. 12, 2758 (2021).
- B. Göbel, A. Mook, J. Henk, and I. Mertig, Antiferromagnetic skyrmion crystals: Generation, topological Hall, and topological spin Hall effect, Phys. Rev. B 96, 060406(R) (2017).
- B. Göbel, A. Mook, J. Henk, and I. Mertig, The family of topological Hall effects for electrons in skyrmion crystals, Eur. Phys. J. B 91, 179 (2018).
- B. Göbel, A. Schäffer, J. Berakdar, I. Mertig, and S. Parkin, Electrical writing, deleting, reading, and moving of magnetic skyrmioniums in a racetrack device, Sci. Rep. 9, 12119 (2019).
- P. K. Sivakumar, B. Göbel, E. Lesne, A. Markou, J. Gidugu, J. M. Taylor, H. Deniz, J. Jena, C. Felser, I. Mertig et al., Topological Hall signatures of two chiral spin textures hosted in a single tetragonal inverse Heusler thin film, ACS Nano 14, 13463 (2020).
- H. Hopf, Über die abbildungen der dreidimensionalen sphäre auf die kugelfläche, Math. Ann. 104, 637 (1931).
- V. E. Korepin and L. D. Faddeev, Quantization of solitons, Theor. Math. Phys. 25, 1039 (1975).
- P. Sutcliffe, Vortex rings in ferromagnets: Numerical simulations of the time-dependent three-dimensional Landau-Lifshitz equation, Phys. Rev. B 76, 184439 (2007).
- P. Sutcliffe, Skyrmion knots in frustrated magnets, Phys. Rev. Lett. 118, 247203 (2017).
- P. Sutcliffe, Hopfions in chiral magnets, J. Phys. A: Math. Theor. 51, 375401 (2018).
- Y. Liu, R. K. Lake, and J. Zang, Binding a hopfion in a chiral magnet nanodisk, Phys. Rev. B 98, 174437 (2018).
- J.-S. B. Tai, I. I. Smalyukh et al., Static Hopf solitons and knotted emergent fields in solid-state noncentrosymmetric magnetic nanostructures, Phys. Rev. Lett. 121, 187201 (2018).
- X. S. Wang, A. Qaiumzadeh, and A. Brataas, Current-driven dynamics of magnetic hopfions, Phys. Rev. Lett. 123, 147203 (2019).
- B. Göbel, C. A. Akosa, G. Tatara, and I. Mertig, Topological Hall signatures of magnetic hopfions, Phys. Rev. Res. 2, 013315 (2020).
- Y. Liu, W. Hou, X. Han, and J. Zang, Three-dimensional dynamics of a magnetic hopfion driven by spin transfer torque, Phys. Rev. Lett. 124, 127204 (2020).
- D. Raftrey and P. Fischer, Field-driven dynamics of magnetic hopfions, Phys. Rev. Lett. 127, 257201 (2021).
- N. Kent, N. Reynolds, D. Raftrey, I. T. Campbell, S. Virasawmy, S. Dhuey, R. V. Chopdekar, A. Hierro-Rodriguez, A. Sorrentino, E. Pereiro et al., Creation and observation of hopfions in magnetic multilayer systems, Nat. Commun. 12, 1562 (2021).
- F. N. Rybakov, N. S. Kiselev, A. B. Borisov, L. Döring, C. Melcher, and S. Blügel, Magnetic hopfions in solids, APL Mater. 10, 111113 (2022).
- D. Popadiuk, E. Tartakovskaya, M. Krawczyk, and K. Guslienko, Emergent magnetic field and nonzero gyrovector of the toroidal magnetic hopfion, Phys. Status Solidi Rapid Res. Lett. 17, 2300131 (2023).
- F. Zheng, N. S. Kiselev, F. N. Rybakov, L. Yang, W. Shi, S. Blügel, and R. E. Dunin-Borkowski, Hopfion rings in a cubic chiral magnet, Nature (London) 623, 718 (2023).
- X. Zhang, J. Xia, Y. Zhou, D. Wang, X. Liu, W. Zhao, and M. Ezawa, Control and manipulation of a magnetic skyrmionium in nanostructures, Phys. Rev. B 94, 094420 (2016).
- S. Zhang, F. Kronast, G. van der Laan, and T. Hesjedal, Real-space observation of skyrmionium in a ferromagnet-magnetic topological insulator heterostructure, Nano Lett. 18, 1057 (2018).
- D. Wolf, N. Biziere, S. Sturm, D. Reyes, T. Wade, T. Niermann, J. Krehl, B. Warot-Fonrose, B. Büchner, E. Snoeck et al., Holographic vector field electron tomography of three-dimensional nanomagnets, Commun. Phys. 2, 87 (2019).
- P. A. Midgley and R. E. Dunin-Borkowski, Electron tomography and holography in materials science, Nat. Mater. 8, 271 (2009).
- A. Hierro-Rodriguez, C. Quirós, A. Sorrentino, L. M. Álvarez-Prado, J. I. Martín, J. M. Alameda, S. McVitie, E. Pereiro, M. Velez, and S. Ferrer, Revealing 3D magnetization of thin films with soft x-ray tomography: Magnetic singularities and topological charges, Nat. Commun. 11, 6382 (2020).
- D. Wolf, S. Schneider, U. K. Rößler, A. Kovács, M. Schmidt, R. E. Dunin-Borkowski, B. Büchner, B. Rellinghaus, and A. Lubk, Unveiling the three-dimensional magnetic texture of skyrmion tubes, Nat. Nanotechnol. 17, 250 (2022).
- S. Seki, M. Suzuki, M. Ishibashi, R. Takagi, N. Khanh, Y. Shiota, K. Shibata, W. Koshibae, Y. Tokura, and T. Ono, Direct visualization of the three-dimensional shape of skyrmion strings in a noncentrosymmetric magnet, Nat. Mater. 21, 181 (2022).
- F. S. Yasin, J. Masell, Y. Takahashi, T. Akashi, N. Baba, K. Karube, D. Shindo, T. Arima, Y. Taguchi, Y. Tokura et al., Bloch point quadrupole constituting hybrid topological strings revealed with electron holographic vector field tomography, Adv. Mater. 36, 2311737 (2024).
- M. Winterott and S. Lounis, Unlocking hidden potential in electron holography of non-collinear spin textures, arXiv:2502.18949.
- G. Gubbiotti, A. Barman, S. Ladak, C. Bran, D. Grundler, M. Huth, H. Plank, G. Schmidt, S. Van Dijken, R. Streubel et al., 2025 roadmap on 3D nano-magnetism, J. Phys.: Condens. Matter 37, 143502 (2025).
- L. S. Levitov, Y. V. Nazarov, and G. M. Éliashberg, Magnetoelectric effects in conductors with mirror isomer symmetry, Sov. Phys. JETP 61, 133 (1985).
- T. Yoda, T. Yokoyama, and S. Murakami, Current-induced orbital and spin magnetizations in crystals with helical structure, Sci. Rep. 5, 12024 (2015).
- T. Yoda, T. Yokoyama, and S. Murakami, Orbital Edelstein effect as a condensed-matter analog of solenoids, Nano Lett. 18, 916 (2018).
- D. Go, J.-P. Hanke, P. M. Buhl, F. Freimuth, G. Bihlmayer, H.-W. Lee, Y. Mokrousov, and S. Blügel, Toward surface orbitronics: Giant orbital magnetism from the orbital Rashba effect at the surface of -metals, Sci. Rep. 7, 46742 (2017).
- L. Salemi, M. Berritta, A. K. Nandy, and P. M. Oppeneer, Orbitally dominated Rashba-Edelstein effect in noncentrosymmetric antiferromagnets, Nat. Commun. 10, 5381 (2019).
- A. Johansson, B. Göbel, J. Henk, M. Bibes, and I. Mertig, Spin and orbital Edelstein effects in a two-dimensional electron gas: Theory and application to interfaces, Phys. Rev. Res. 3, 013275 (2021).
- Y. Liu, J. Xiao, J. Koo, and B. Yan, Chirality-driven topological electronic structure of DNA-like materials, Nat. Mater. 20, 638 (2021).
- B. Kim, D. Shin, S. Namgung, N. Park, K.-W. Kim, and J. Kim, Optoelectronic manifestation of orbital angular momentum driven by chiral hopping in helical Se chains, ACS Nano 17, 18873 (2023).
- A. El Hamdi, J.-Y. Chauleau, M. Boselli, C. Thibault, C. Gorini, A. Smogunov, C. Barreteau, S. Gariglio, J.-M. Triscone, and M. Viret, Observation of the orbital inverse Rashba–Edelstein effect, Nat. Phys. 19, 1855 (2023).
- K. Hagiwara, Y.-J. Chen, D. Go, X. L. Tan, S. Grytsiuk, K.-H. O. Yang, G.-J. Shu, J. Chien, Y.-H. Shen, X.-L. Huang et al., Orbital topology of chiral crystals for orbitronics, Adv. Mater. 37, 2418040 (2025).
- J. M. Lee, M. J. Park, and H.-W. Lee, Orbital Edelstein effect of electronic itinerant orbital motion at edges, Phys. Rev. B 110, 134436 (2024).
- B. Göbel, L. Schimpf, and I. Mertig, Chirality-induced orbital Edelstein effect in an analytically solvable model, Phys. Rev. Res. 7, 033180 (2025).
- O. Busch, F. Ziolkowski, B. Göbel, I. Mertig, and J. Henk, Nonlinear spin and orbital Rashba-Edelstein effects induced by a femtosecond laser pulse Simulations for Au(001), Phys. Rev. Res. 7, 043023 (2025).
- B. Göbel, I. Mertig, and S. Lounis, Chirality-induced selectivity of angular momentum by orbital Edelstein effect in carbon nanotubes, Commun. Phys. 8, 395 (2025).
- S. Zhang and Z. Yang, Intrinsic spin and orbital angular momentum Hall effect, Phys. Rev. Lett. 94, 066602 (2005).
- B. A. Bernevig, T. L. Hughes, and S.-C. Zhang, Orbitronics: The intrinsic orbital current in -doped silicon, Phys. Rev. Lett. 95, 066601 (2005).
- H. Kontani, T. Tanaka, D. S. Hirashima, K. Yamada, and J. Inoue, Giant intrinsic spin and orbital Hall effects in (, Rh, Mo), Phys. Rev. Lett. 100, 096601 (2008).
- T. Tanaka, H. Kontani, M. Naito, T. Naito, D. S. Hirashima, K. Yamada, and J. Inoue, Intrinsic spin Hall effect and orbital Hall effect in and transition metals, Phys. Rev. B 77, 165117 (2008).
- H. Kontani, T. Tanaka, D. S. Hirashima, K. Yamada, and J. Inoue, Giant orbital Hall effect in transition metals: Origin of large spin and anomalous Hall effects, Phys. Rev. Lett. 102, 016601 (2009).
- D. Go, D. Jo, C. Kim, and H.-W. Lee, Intrinsic spin and orbital Hall effects from orbital texture, Phys. Rev. Lett. 121, 086602 (2018).
- A. Pezo, D. Garcia Ovalle, and A. Manchon, Orbital Hall effect in crystals: Interatomic versus intra-atomic contributions, Phys. Rev. B 106, 104414 (2022).
- L. M. Canonico, T. P. Cysne, A. Molina-Sanchez, R. B. Muniz, and T. G. Rappoport, Orbital Hall insulating phase in transition metal dichalcogenide monolayers, Phys. Rev. B 101, 161409(R) (2020).
- T. P. Cysne, S. Bhowal, G. Vignale, and T. G. Rappoport, Orbital Hall effect in bilayer transition metal dichalcogenides: From the intra-atomic approximation to the Bloch states orbital magnetic moment approach, Phys. Rev. B 105, 195421 (2022).
- L. Salemi and P. M. Oppeneer, Theory of magnetic spin and orbital Hall and Nernst effects in bulk ferromagnets, Phys. Rev. B 106, 024410 (2022).
- O. Busch, I. Mertig, and B. Göbel, Orbital Hall effect and orbital edge states caused by electrons, Phys. Rev. Res. 5, 043052 (2023).
- Y.-G. Choi, D. Jo, K.-H. Ko, D. Go, K.-H. Kim, H. G. Park, C. Kim, B.-C. Min, G.-M. Choi, and H.-W. Lee, Observation of the orbital Hall effect in a light metal Ti, Nature (London) 619, 52 (2023).
- I. Lyalin, S. Alikhah, M. Berritta, P. M. Oppeneer, and R. K. Kawakami, Magneto-optical detection of the orbital Hall effect in chromium, Phys. Rev. Lett. 131, 156702 (2023).
- O. Busch, F. Ziolkowski, B. Göbel, I. Mertig, and J. Henk, Ultrafast orbital Hall effect in metallic nanoribbons, Phys. Rev. Res. 6, 013208 (2024).
- B. Göbel and I. Mertig, Orbital Hall effect accompanying quantum Hall effect: Landau levels cause orbital polarized edge currents, Phys. Rev. Lett. 133, 146301 (2024).
- B. Göbel, L. Schimpf, and I. Mertig, Topological orbital Hall effect caused by skyrmions and antiferromagnetic skyrmions, Commun. Phys. 8, 17 (2025).
- M. d. S. Dias, J. Bouaziz, M. Bouhassoune, S. Blügel, and S. Lounis, Chirality-driven orbital magnetic moments as a new probe for topological magnetic structures, Nat. Commun. 7, 13613 (2016).
- F. R. Lux, F. Freimuth, S. Blügel, and Y. Mokrousov, Engineering chiral and topological orbital magnetism of domain walls and skyrmions, Commun. Phys. 1, 60 (2018).
- B. Göbel, A. Mook, J. Henk, and I. Mertig, Magnetoelectric effect and orbital magnetization in skyrmion crystals: Detection and characterization of skyrmions, Phys. Rev. B 99, 060406(R) (2019).
- J. Barker and O. A. Tretiakov, Static and dynamical properties of antiferromagnetic skyrmions in the presence of applied current and temperature, Phys. Rev. Lett. 116, 147203 (2016).
- X. Zhang, Y. Zhou, and M. Ezawa, Magnetic bilayer-skyrmions without skyrmion Hall effect, Nat. Commun. 7, 10293 (2016).
- X. Zhang, Y. Zhou, and M. Ezawa, Antiferromagnetic skyrmion: Stability, creation and manipulation, Sci. Rep. 6, 24795 (2016).
- W. Legrand, D. Maccariello, F. Ajejas, S. Collin, A. Vecchiola, K. Bouzehouane, N. Reyren, V. Cros, and A. Fert, Room-temperature stabilization of antiferromagnetic skyrmions in synthetic antiferromagnets, Nat. Mater. 19, 34 (2020).
- J. Whitehead, An expression of Hopf's invariant as an integral, Proc. Natl. Acad. Sci. USA 33, 117 (1947).
- F. Wilczek and A. Zee, Linking numbers, spin, and statistics of solitons, Phys. Rev. Lett. 51, 2250 (1983).
- R. Knapman, M. Azhar, A. Pignedoli, L. Gallard, R. Hertel, J. Leliaert, and K. Everschor-Sitte, Numerical calculation of the Hopf index for three-dimensional magnetic textures, Phys. Rev. B 111, 134408 (2025).
- K. Ohgushi, S. Murakami, and N. Nagaosa, Spin anisotropy and quantum Hall effect in the kagomé lattice: Chiral spin state based on a ferromagnet, Phys. Rev. B 62, R6065 (2000).
- K. Hamamoto, M. Ezawa, and N. Nagaosa, Quantized topological Hall effect in skyrmion crystal, Phys. Rev. B 92, 115417 (2015).
- B. Göbel, A. Mook, J. Henk, and I. Mertig, Unconventional topological Hall effect in skyrmion crystals caused by the topology of the lattice, Phys. Rev. B 95, 094413 (2017).
- G. Yin, Y. Liu, Y. Barlas, J. Zang, and R. K. Lake, Topological spin Hall effect resulting from magnetic skyrmions, Phys. Rev. B 92, 024411 (2015).
- M.-C. Chang and Q. Niu, Berry phase, hyperorbits, and the Hofstadter spectrum: Semiclassical dynamics in magnetic Bloch bands, Phys. Rev. B 53, 7010 (1996).
- P. Oppeneer, Magneto-optical spectroscopy in the valence-band energy regime: Relationship to the magnetocrystalline anisotropy, J. Magn. Magn. Mater. 188, 275 (1998).
- D. Xiao, J. Shi, and Q. Niu, Berry phase correction to electron density of states in solids, Phys. Rev. Lett. 95, 137204 (2005).
- T. Thonhauser, D. Ceresoli, D. Vanderbilt, and R. Resta, Orbital magnetization in periodic insulators, Phys. Rev. Lett. 95, 137205 (2005).
- D. Ceresoli, T. Thonhauser, D. Vanderbilt, and R. Resta, Orbital magnetization in crystalline solids: Multi-band insulators, Chern insulators, and metals, Phys. Rev. B 74, 024408 (2006).
- A. Raoux, F. Piéchon, J.-N. Fuchs, and G. Montambaux, Orbital magnetism in coupled-bands models, Phys. Rev. B 91, 085120 (2015).
- B. Göbel, A. Mook, J. Henk, and I. Mertig, Signatures of lattice geometry in quantum and topological Hall effect, New J. Phys. 19, 063042 (2017).
- L. Onsager, Interpretation of the de Haas–van Alphen effect, London Edinburgh Dublin Philos. Mag. J. Sci. 43, 1006 (1952).
- Data are provided for figures shown in this paper at Zenodo (2025), doi: 10.5281/zenodo.15609600.