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Evidence of a Kondo lattice quantum critical point and of non-Fermi liquid behavior in the intercalated layered system V5S8

Hancheng Yang1,2, Hicham Moutaabbid1, Benoît Baptiste1, David Hrabovsky3, Andrea Gauzzi1, and Yannick Klein1,*

  • 1IMPMC, Sorbonne Université, CNRS, MNHN, 4 place Jussieu, 75005 Paris, France
  • 2Department of Physics, Zhejiang University, 310058 Hangzhou, China
  • 3Center of Low-Temperature Physical Measurements, Sorbonne Université, 4 place Jussieu, 75005 Paris, France

  • *Contact author: yannick.klein@sorbonne-universite.fr

Phys. Rev. B 111, L241115 – Published 30 June, 2025

DOI: https://doi.org/10.1103/s3zf-rzvz

Abstract

By means of a specific heat, susceptibility, and high-pressure electrical resistivity study, we show that the local magnetic moments of the intercalated V ions in V5S8 realize a prototype of Kondo lattice system, where an antiferromagnetic order of the moments coexists with a Fermi liquid in the VS2 layers with intermediate heavy fermion properties. Our data analysis suggests a simultaneous suppression of Fermi-liquid behavior and of antiferromagnetic order at a critical pressure, Pc=10 GPa, the signature of a quantum critical point. This result supports a Kondo lattice scenario and raises the question whether, in the paramagnetic phase at higher pressures, the heavy quasiparticles survive or form a non-Fermi liquid phase governed by the Kondo interaction.

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