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    Orbital selectivity and metal-insulator crossovers in La1+xSr1−xNiO4 (0≤x≤1)

    L. Craco

    Phys. Rev. B 111, 235126 – Published 13 June, 2025

    DOI: https://doi.org/10.1103/rzmq-xtym

    Abstract

    Based on density functional plus dynamical mean-field theory (DFT + DMFT) calculations, we explore the electronic reconstruction of La1+xSr1−xNiO4(0≤x≤1). We show how Mott localization manifests itself due to sizable electron correlation effects in the eg-shell one-particle spectral functions. Our results upon electron-doping the LaSrNiO4 layered compound provide a many-particle interpretation for the tenacious insulating behavior seen in experiments. Our findings call for future theory and experimental investigations to validate or rule out the proximity to marginal Fermi liquidness as the prominent candidate for pseudogapped transport properties of pressurized LaSrNiO4.

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