- Letter
- Open Access
Triangular Heisenberg antiferromagnet in a magnetic field
Phys. Rev. B 113, L241114 – Published 18 June, 2026
DOI: https://doi.org/10.1103/rwhz-jf5b
Abstract
The behavior of the paradigmatic triangular lattice Heisenberg antiferromagnet in a magnetic field remains unsettled despite decades of study. We map out the phase diagram using three complementary approaches, including self-consistent nonlinear spin-wave theory, density-matrix renormalization group, and variational Monte Carlo. This combined analysis resolves the competition among different field-induced magnetic orders and magnetization plateaus across the classically frustrated parameter range. In particular, there is a finite range in the parameter regime around in which (i) upon the application of the external field, the gapless quantum spin liquid acquires a finite density of monopoles, and (ii) by further increasing the field, two plateaus are clearly obtained at and . We discuss the experimental importance of the consecutive magnetization plateau transitions as a signature of an underlying quantum spin-liquid phase.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (59)
- Introduction to Frustrated Magnetism: Materials, Experiments, Theory, edited by C. Lacroix, P. Mendels, and F. Mila, Springer Series in Solid-State Sciences, Vol. 164 (Springer, Berlin, 2011).
- G. Wannier, Antiferromagnetism. The triangular Ising net, Phys. Rev. 79, 357 (1950).
- B. Metcalf, Phase diagram of a nearest neighbor triangular antiferromagnet in an external field, Phys. Lett. A 45, 1 (1973).
- B. Metcalf, Ground state spin orderings of the triangular Ising model with the nearest and next nearest neighbor interaction, Phys. Lett. A 46, 325 (1974).
- O. Bradley, C. Feng, R. T. Scalettar, and R. R. Singh, Robustness of entropy plateaus: A case study of triangular Ising antiferromagnets, Phys. Rev. B 100, 064414 (2019).
- H. Nishimori and S. Miyashita, Magnetization process of the spin-1/2 antiferromagnetic Ising-like Heisenberg model on the triangular lattice, J. Phys. Soc. Jpn. 55, 4448 (1986).
- A. Chubukov and D. Golosov, Quantum theory of an antiferromagnet on a triangular lattice in a magnetic field, J. Phys.: Condens. Matter 3, 69 (1991).
- H. Kawamura and S. Miyashita, Phase transition of the Heisenberg antiferromagnet on the triangular lattice in a magnetic field, J. Phys. Soc. Jpn. 54, 4530 (1985).
- M. Gvozdikova, P. Melchy, and M. Zhitomirsky, Magnetic phase diagrams of classical triangular and kagome antiferromagnets, J. Phys.: Condens. Matter 23, 164209 (2011).
- L. Seabra, T. Momoi, P. Sindzingre, and N. Shannon, Phase diagram of the classical Heisenberg antiferromagnet on a triangular lattice in an applied magnetic field, Phys. Rev. B 84, 214418 (2011).
- M. Takigawa and F. Mila, Magnetization plateaus, in Introduction to Frustrated Magnetism: Materials, Experiments, Theory (Springer, 2011), Vol. 164, pp. 241–267.
- O. A. Starykh, Unusual ordered phases of highly frustrated magnets: A review, Rep. Prog. Phys. 78, 052502 (2015).
- A. Honecker, J. Schulenburg, and J. Richter, Magnetization plateaus in frustrated antiferromagnetic quantum spin models, J. Phys.: Condens. Matter 16, S749 (2004).
- T. Ono, H. Tanaka, H. Aruga Katori, F. Ishikawa, H. Mitamura, and T. Goto, Magnetization plateau in the frustrated quantum spin system , Phys. Rev. B 67, 104431 (2003).
- Y. Shirata, H. Tanaka, A. Matsuo, and K. Kindo, Experimental realization of a spin-1/2 triangular-lattice Heisenberg antiferromagnet, Phys. Rev. Lett. 108, 057205 (2012).
- L. Savary and L. Balents, Quantum spin liquids: A review, Rep. Prog. Phys. 80, 016502 (2017).
- J. Knolle and R. Moessner, A field guide to spin liquids, Annu. Rev. Condens. Matter Phys. 10, 451 (2019).
- C. Broholm, R. J. Cava, S. Kivelson, D. Nocera, M. Norman, and T. Senthil, Quantum spin liquids, Science 367, eaay0668 (2020).
- K. Kanoda and R. Kato, Mott physics in organic conductors with triangular lattices, Annu. Rev. Condens. Matter Phys. 2, 167 (2011).
- Z. Zhu and S. R. White, Spin liquid phase of the Heisenberg model on the triangular lattice, Phys. Rev. B 92, 041105(R) (2015).
- S.-S. Gong, W. Zheng, M. Lee, Y.-M. Lu, and D. N. Sheng, Chiral spin liquid with spinon Fermi surfaces in the spin- triangular Heisenberg model, Phys. Rev. B 100, 241111(R) (2019).
- Z. Zhu, P. A. Maksimov, S. R. White, and A. L. Chernyshev, Topography of spin liquids on a triangular lattice, Phys. Rev. Lett. 120, 207203 (2018).
- M. Drescher, L. Vanderstraeten, R. Moessner, and F. Pollmann, Dynamical signatures of symmetry-broken and liquid phases in an Heisenberg antiferromagnet on the triangular lattice, Phys. Rev. B 108, L220401 (2023).
- A. O. Scheie, Y. Kamiya, H. Zhang, S. Lee, A. J. Woods, M. O. Ajeesh, M. G. Gonzalez, B. Bernu, J. W. Villanova, J. Xing, Q. Huang, Q. Zhang, J. Ma, E. S. Choi, D. M. Pajerowski, H. Zhou, A. S. Sefat, S. Okamoto, T. Berlijn, L. Messio, et al., Nonlinear magnons and exchange Hamiltonians of the delafossite proximate quantum spin liquid candidates and , Phys. Rev. B 109, 014425 (2024).
- Y. Shen, Y.-D. Li, H. Wo, Y. Li, S. Shen, B. Pan, Q. Wang, H. C. Walker, P. Steffens, M. Boehm, Y. Hao, D. L. Quintero-Castro, L. W. Harriger, M. D. Frontzek, L. Hao, S. Meng, Q. Zhang, G. Chen, and J. Zhao, Evidence for a spinon Fermi surface in a triangular-lattice quantum-spin-liquid candidate, Nature (London) 540, 559 (2016).
- P. Anderson, Resonating valence bonds: A new kind of insulator? Mater. Res. Bull. 8, 153 (1973).
- W.-J. Hu, S.-S. Gong, W. Zhu, and D. N. Sheng, Competing spin-liquid states in the spin- Heisenberg model on the triangular lattice, Phys. Rev. B 92, 140403(R) (2015).
- Y. Iqbal, W.-J. Hu, R. Thomale, D. Poilblanc, and F. Becca, Spin liquid nature in the Heisenberg triangular antiferromagnet, Phys. Rev. B 93, 144411 (2016).
- F. Ferrari and F. Becca, Dynamical structure factor of the Heisenberg model on the triangular lattice: Magnons, spinons, and gauge fields, Phys. Rev. X 9, 031026 (2019).
- T. Tang, B. Moritz, and T. P. Devereaux, Spectra of a gapped quantum spin liquid with a strong chiral excitation on the triangular lattice, Phys. Rev. B 106, 064428 (2022).
- A. O. Scheie, E. A. Ghioldi, J. Xing, J. A. M. Paddison, N. E. Sherman, M. Dupont, L. D. Sanjeewa, S. Lee, A. J. Woods, D. Abernathy, D. M. Pajerowski, T. J. Williams, S.-S. Zhang, L. O. Manuel, A. E. Trumper, C. D. Pemmaraju, A. S. Sefat, D. S. Parker, T. P. Devereaux, R. Movshovich, et al., Proximate spin liquid and fractionalization in the triangular antiferromagnet , Nat. Phys. 20, 74 (2024).
- T. Xie, A. A. Eberharter, J. Xing, S. Nishimoto, M. Brando, P. Khanenko, J. Sichelschmidt, A. A. Turrini, D. G. Mazzone, P. G. Naumov, L. D. Sanjeewa, N. Harrison, A. S. Sefat, B. Normand, A. M. Läuchli, A. Podlesnyak, and S. E. Nikitin, Complete field-induced spectral response of the spin-1/2 triangular-lattice antiferromagnet , npj Quantum Mater. 8, 48 (2023).
- A. Scheie, M. Lee, K. Wang, P. Laurell, E. Choi, D. Pajerowski, Q. Zhang, J. Ma, H. Zhou, S. Lee, et al., Spectrum and low-energy gap in triangular quantum spin liquid , arXiv:2406.17773.
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/rwhz-jf5b for details of the linear and nonlinear spin wave theories, and the determination of phase boundaries.
- T. Jolicoeur, E. Dagotto, E. Gagliano, and S. Bacci, Ground-state properties of the = 1/2 Heisenberg antiferromagnet on a triangular lattice, Phys. Rev. B 42, 4800 (1990).
- A. V. Chubukov and T. Jolicoeur, Order-from-disorder phenomena in Heisenberg antiferromagnets on a triangular lattice, Phys. Rev. B 46, 11137 (1992).
- D. A. Huse and V. Elser, Simple variational wave functions for two-dimensional Heisenberg spin-½ antiferromagnets, Phys. Rev. Lett. 60, 2531 (1988).
- T. Coletta, T. A. Tóth, K. Penc, and F. Mila, Semiclassical theory of the magnetization process of the triangular lattice Heisenberg model, Phys. Rev. B 94, 075136 (2016).
- M. Ye and A. V. Chubukov, Quantum phase transitions in the Heisenberg triangular antiferromagnet in a magnetic field, Phys. Rev. B 95, 014425 (2017).
- M. Ye and A. V. Chubukov, Half-magnetization plateau in a Heisenberg antiferromagnet on a triangular lattice, Phys. Rev. B 96, 140406(R) (2017).
- S. R. White, Density matrix formulation for quantum renormalization groups, Phys. Rev. Lett. 69, 2863 (1992).
- J. Hauschild, J. Unfried, S. Anand, B. Andrews, M. Bintz, U. Borla, S. Divic, M. Drescher, J. Geiger, M. Hefel, K. Hémery, W. Kadow, J. Kemp, N. Kirchner, V. S. Liu, G. Möller, D. Parker, M. Rader, A. Romen, S. Scalet, et al., Tensor network Python (TeNPy) version 1, SciPost Phys. Codebases 41 (2024).
- F. Becca and S. Sorella, Quantum Monte Carlo Approaches for Correlated Systems (Cambridge University Press, Cambridge, UK, 2017).
- R. Yadav, S. Rachel, L. Hozoi, J. van den Brink, and G. Jackeli, Strain- and pressure-tuned magnetic interactions in honeycomb Kitaev materials, Phys. Rev. B 98, 121107(R) (2018).
- P. Sakrikar, B. Shen, E. H. T. Poldi, F. Bahrami, X. Hu, E. M. Kenney, Q. Wang, K. W. Fruhling, C. Wang, R. Gupta, R. Khasanov, H. Luetkens, S. A. Calder, A. A. Aczel, G. Fabbris, R. J. Hemley, K. W. Plumb, Y. Ran, P. Gegenwart, A. A. Tsirlin, et al., Pressure tuning of competing interactions on a honeycomb lattice, Nat. Commun. 16, 4712 (2025).
- B. P. Belbase, A. Unnikrishnan, S. Feng, E. S. Choi, J. Knolle, and A. Banerjee, Finite spinon density-of-states in triangular-lattice delafossite , arXiv:2504.05436.
- D. Sellmann, X.-F. Zhang, and S. Eggert, Phase diagram of the antiferromagnetic XXZ model on the triangular lattice, Phys. Rev. B 91, 081104(R) (2015).
- D. Yamamoto, G. Marmorini, and I. Danshita, Quantum phase diagram of the triangular-lattice XXZ model in a magnetic field, Phys. Rev. Lett. 112, 127203 (2014).
- L. Seabra and N. Shannon, Competition between supersolid phases and magnetization plateaus in the frustrated easy-axis antiferromagnet on a triangular lattice, Phys. Rev. B 83, 134412 (2011).
- S. Hu, W. Zhu, S. Eggert, and Y.-C. He, Dirac spin liquid on the spin- triangular Heisenberg antiferromagnet, Phys. Rev. Lett. 123, 207203 (2019).
- Y.-C. He, M. P. Zaletel, M. Oshikawa, and F. Pollmann, Signatures of Dirac cones in a DMRG study of the kagome Heisenberg model, Phys. Rev. X 7, 031020 (2017).
- S. Budaraju et al., Field induced monopole condensate in the triangular Heisenberg model in a magnetic field (unpublished).
- X.-Y. Song, C. Wang, A. Vishwanath, and Y.-C. He, Unifying description of competing orders in two-dimensional quantum magnets, Nat. Commun. 10, 4254 (2019).
- S. Budaraju, A. Parola, Y. Iqbal, F. Becca, and D. Poilblanc, Monopole excitations in the Dirac spin liquid on the triangular lattice, Phys. Rev. B 111, 125150 (2025).
- X.-Y. Song, Y.-C. He, A. Vishwanath, and C. Wang, From spinon band topology to the symmetry quantum numbers of monopoles in Dirac spin liquids, Phys. Rev. X 10, 011033 (2020).
- Y. Ran, W.-H. Ko, P. A. Lee, and X.-G. Wen, Spontaneous spin ordering of a Dirac spin liquid in a magnetic field, Phys. Rev. Lett. 102, 047205 (2009).
- A. Keselman, X. Xu, H. Zhang, C. D. Batista, and O. A. Starykh, triangular lattice antiferromagnet in a magnetic field, arXiv:2512.02150.
- W. O. Wang, U. F. P. Seifert, O. A. Starykh, and L. Balents, Chirality and quasi-long-range order in finite-flux Gutzwiller states for magnetized frustrated magnets, arXiv:2601.14458.
- T. Bader, S. Feng, S. Budaraju, B. Federico, J. Knolle, and F. Pollmann, Triangular Heisenberg antiferromagnet in a magnetic field [Dataset], Zenodo, 2026, https://doi.org/10.5281/zenodo.20510149.