Comparative study of terbium tellurides and
Phys. Rev. B 112, 094434 – Published 17 September, 2025
DOI: https://doi.org/10.1103/rm6p-8hzd
Abstract
Two terbium tellurides, and , were studied by means of thermodynamics, ultrafast pump-probe spectroscopy, and torque magnetometry. While the crystal structure and some physical properties of were established previously, the crystal structure of is reported based on the low-temperature (100 K) single crystal x-ray diffraction experiment. crystallizes in orthorhombic Cmcm space group with , , , , and . In contrast to , which experiences three successive magnetic phase transitions, orders antiferromagnetically in two steps at K and K, both readily suppressed by an external magnetic field. The third transition in is due to the interaction of the magnetic subsystem with the charge density waves. The interaction of magnetic and electronic subsystems in has been revealed by the pump probe. Torque measurements of show that the magnetic moments of Tb are oriented predominantly in the plane at high temperatures and switch to the axis at low temperatures. In , the magnetic moments of Tb are oriented predominantly in the plane at low temperatures.