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    Field-rigid Ising antiferromagnetism with giant metamagnetic transition fields in van der Waals UOTe

    Zackary Rehfuss1, Shannon Gould1, Joanna Blawat2, Christopher Broyles1, Qiaozhi Xu1, Yiqing Hao3, Huibo Cao3, Thao Dinh4, Suyang Xu4 et al.

    Dave Graf5, John Singleton2, and Sheng Ran1

    Phys. Rev. B 114, 144422 – Published 24 September, 2026

    DOI: https://doi.org/10.1103/r9cs-6qj5

    Abstract

    van der Waals antiferromagnets provide a route to thickness-controlled magnetic order, but few combine high-temperature Ising order with conducting, correlated, and topological electronic structure. Here we show that UOTe realizes this combination. Magnetic susceptibility reveals a strongly anisotropic paramagnetic response, while neutron diffraction establishes c-axis antiferromagnetic order below TN≈150K with an order-parameter exponent β=0.14, close to the two-dimensional Ising value. Torque magnetometry further shows that the ordered state remains well described by a uniaxial antiferromagnet below the high-field metamagnetic transition. Pulsed-field magnetization up to 73T shows that the ordered state survives to very large fields applied along the c axis before entering a broad metamagnetic regime that begins near 50T and remains unsaturated at the highest measured field. Angle-dependent proximity detector oscillator measurements show that the metamagnetic instability is set by the field component along the ordered moment direction, providing direct evidence for Ising-like field rigidity. UOTe therefore establishes a field-rigid Ising antiferromagnet with giant metamagnetic transition fields in a compensated van der Waals metal, where high-temperature c-axis order, quasi-two-dimensional magnetic criticality, Kondo-associated uranium 5f hybridization, metallic transport, and symmetry-enabled topology coexist in a single material.

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