Field-rigid Ising antiferromagnetism with giant metamagnetic transition fields in van der Waals UOTe
Phys. Rev. B 114, 144422 – Published 24 September, 2026
DOI: https://doi.org/10.1103/r9cs-6qj5
Abstract
van der Waals antiferromagnets provide a route to thickness-controlled magnetic order, but few combine high-temperature Ising order with conducting, correlated, and topological electronic structure. Here we show that UOTe realizes this combination. Magnetic susceptibility reveals a strongly anisotropic paramagnetic response, while neutron diffraction establishes -axis antiferromagnetic order below with an order-parameter exponent , close to the two-dimensional Ising value. Torque magnetometry further shows that the ordered state remains well described by a uniaxial antiferromagnet below the high-field metamagnetic transition. Pulsed-field magnetization up to shows that the ordered state survives to very large fields applied along the axis before entering a broad metamagnetic regime that begins near and remains unsaturated at the highest measured field. Angle-dependent proximity detector oscillator measurements show that the metamagnetic instability is set by the field component along the ordered moment direction, providing direct evidence for Ising-like field rigidity. UOTe therefore establishes a field-rigid Ising antiferromagnet with giant metamagnetic transition fields in a compensated van der Waals metal, where high-temperature -axis order, quasi-two-dimensional magnetic criticality, Kondo-associated uranium hybridization, metallic transport, and symmetry-enabled topology coexist in a single material.